Wen Kaichuan, Cao Yu, Gu Lianghui, Wang Saixue, Qian Dongmin, Wang Jingmin, Kuang Zhiyuan, Luo Mengyi, Wang Gang, Guan Shuzhen, Li Mengmeng, Yang Heng, Xing Guichuan, Wang Nana, Zhu Lin, Peng Qiming, Huang Wei, Wang Jianpu
Key Laboratory of Flexible Electronics (KLOFE), Institute of Advanced Materials (IAM) & School of Flexible Electronics (Future Technologies), Nanjing Tech University (NanjingTech), 30 South Puzhu Road, Nanjing, 211816, China.
Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China.
Adv Mater. 2023 Nov;35(44):e2303144. doi: 10.1002/adma.202303144. Epub 2023 Sep 21.
Realization of electrically pumped laser diodes based on solution-processed semiconductors is a long-standing challenge. Metal halide perovskites have shown great potential toward this goal due to their excellent optoelectronic properties. Continuous-wave (CW) optically pumped lasing in a real electroluminescent device represents a key step to current-injection laser diodes, but it has not yet been realized. This is mainly due to the challenge of incorporating a resonant cavity into an efficient light-emitting diode (LED) able to sustain intensive carrier injection. Here, CW lasing is reported in an efficient perovskite LED with an integrated distributed feedback resonator, which shows a low lasing threshold of 220 W cm at 110 K. Importantly, the LED works well at a current density of 330 A cm , indicating the carrier injection rate already exceeds the threshold of optically pumping. The results suggest that electrically pumped perovskite laser diodes can be achieved once the Joule heating issue is overcome.
基于溶液处理半导体实现电泵浦激光二极管是一个长期存在的挑战。金属卤化物钙钛矿因其优异的光电特性,在实现这一目标方面展现出了巨大潜力。在实际的电致发光器件中实现连续波(CW)光泵浦激光是迈向电流注入激光二极管的关键一步,但尚未实现。这主要是由于将谐振腔集成到能够承受高强度载流子注入的高效发光二极管(LED)中存在挑战。在此,报道了在具有集成分布式反馈谐振器的高效钙钛矿LED中实现了连续波激光,其在110K时显示出220W/cm²的低激光阈值。重要的是,该LED在330A/cm²的电流密度下工作良好,表明载流子注入速率已经超过了光泵浦阈值。结果表明,一旦克服焦耳热问题,就可以实现电泵浦钙钛矿激光二极管。