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在纳秒泵浦下具有低阈值的光泵浦CsPbBr激光器中的电可切换增益

Electrically-Switchable Gain in Optically Pumped CsPbBr Lasers With Low Threshold at Nanosecond Pumping.

作者信息

Li Yang, Liu Shangpu, Feeney Thomas, Roger Julie, Gholipoor Mohammad, Hu Hang, Zhao Dewei, Howard Ian, Deschler Felix, Lemmer Uli, Paetzold Ulrich W

机构信息

College of Materials Science and Engineering & Engineering Research Center of Alternative Energy Materials and Devices, Ministry of Education, Sichuan University, Chengdu, 610065, China.

Institute of Microstructure Technology, Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1, 76344, Eggenstein-Leopoldshafen, Germany.

出版信息

Small. 2025 Apr;21(13):e2411935. doi: 10.1002/smll.202411935. Epub 2025 Feb 24.

Abstract

Metal halide perovskites hold promise for nonepitaxial laser diodes, yet, continuous-wave (CW) optically pumped (photonic) lasing in CsPbBr remains elusive despite its superior thermal- and photo-stability among the perovskite family. This work reports on CsPbBr vertical cavity surface emitting lasers with low lasing thresholds (1.3 µJ cm ) at nanosecond pumping and remarkable lasing stability. Furthermore, the electrically switchable gain is achieved in CsPbBr electrically assisted optically pumped laser (EAOPL) devices by leveraging ion migration. Applying a small positive DC voltage to the EAOPL device significantly reduces the lasing threshold under nanosecond laser excitation and enhances the cavity mode intensity at CW laser excitation. These findings present a novel strategy, combining a small DC voltage with an electrical pulse, for exploring electrical injection lasing in CsPbBr perovskites.

摘要

金属卤化物钙钛矿有望用于非外延激光二极管,然而,尽管CsPbBr在钙钛矿家族中具有优异的热稳定性和光稳定性,但连续波(CW)光泵浦(光子)激光在CsPbBr中仍难以实现。这项工作报道了具有低激光阈值(1.3 μJ cm)的CsPbBr垂直腔面发射激光器,在纳秒泵浦下具有显著的激光稳定性。此外,通过利用离子迁移,在CsPbBr电辅助光泵浦激光器(EAOPL)器件中实现了电可切换增益。在EAOPL器件上施加一个小的正直流电压,可显著降低纳秒激光激发下的激光阈值,并增强连续波光激发下的腔模强度。这些发现提出了一种将小直流电压与电脉冲相结合的新策略,用于探索CsPbBr钙钛矿中的电注入激光。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ec90/11962692/64dfa795ac85/SMLL-21-2411935-g001.jpg

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