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欠掺杂钕锶镍氧化物无限层超导薄膜中的近藤散射

Kondo scattering in underdoped NdSrNiO infinite-layer superconducting thin films.

作者信息

Shao Ting-Na, Zhang Zi-Tao, Qiao Yu-Jie, Zhao Qiang, Liu Hai-Wen, Chen Xin-Xiang, Jiang Wei-Min, Yao Chun-Li, Chen Xing-Yu, Chen Mei-Hui, Dou Rui-Fen, Xiong Chang-Min, Zhang Guang-Ming, Yang Yi-Feng, Nie Jia-Cai

机构信息

Department of Physics, Beijing Normal University, Beijing100875, China.

State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing100084, China.

出版信息

Natl Sci Rev. 2023 Apr 25;10(11):nwad112. doi: 10.1093/nsr/nwad112. eCollection 2023 Nov.

Abstract

The recent discovery of superconductivity in infinite-layer nickelates generates tremendous research endeavors, but the ground state of their parent compounds is still under debate. Here, we report experimental evidence for the dominant role of Kondo scattering in the underdoped NdSrNiO thin films. A resistivity minimum associated with logarithmic temperature dependence in both longitudinal and Hall resistivities are observed in the underdoped NdSrNiO samples before the superconducting transition. At lower temperatures down to 0.04 K, the resistivities become saturated, following the prediction of the Kondo model. A linear scaling behavior [Formula: see text] between anomalous Hall conductivity [Formula: see text] and conductivity [Formula: see text]is revealed, verifying the dominant Kondo scattering at low temperature. The effect of weak (anti-)localization is found to be secondary. Our experiments can help in clarifying the basic physics in the underdoped NdSrNiO infinite-layer thin films.

摘要

近期在无限层镍酸盐中发现超导性引发了大量的研究工作,但其母体化合物的基态仍存在争议。在此,我们报告了近藤散射在欠掺杂钕锶镍氧化物薄膜中起主导作用的实验证据。在超导转变之前,在欠掺杂的钕锶镍氧化物样品中观察到纵向和霍尔电阻率都存在与对数温度依赖性相关的电阻率最小值。在低至0.04 K的较低温度下,电阻率如近藤模型所预测的那样达到饱和。揭示了反常霍尔电导率[公式:见正文]与电导率[公式:见正文]之间的线性标度行为[公式:见正文],证实了低温下近藤散射的主导地位。发现弱(反)局域化效应是次要的。我们的实验有助于阐明欠掺杂钕锶镍氧化物无限层薄膜中的基本物理现象。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e3f3/10561711/ced9ea6657a7/nwad112fig1.jpg

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