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热导率的声子量子:模拟和测量所估计的是同一量值吗?

The phonon quantum of thermal conductance: Are simulations and measurements estimating the same quantity?

作者信息

Polanco Carlos A, van Roekeghem Ambroise, Brisuda Boris, Saminadayar Laurent, Bourgeois Olivier, Mingo Natalio

机构信息

Université Grenoble Alpes, CEA, LITEN, 17 rue des Martyrs, Grenoble, France.

Université Grenoble Alpes, CNRS, Grenoble INP, Institut Néel, Grenoble, France.

出版信息

Sci Adv. 2023 Oct 13;9(41):eadi7439. doi: 10.1126/sciadv.adi7439.

DOI:10.1126/sciadv.adi7439
PMID:37831773
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11090371/
Abstract

The thermal conductance quantum is a fundamental quantity in quantum transport theory. However, two decades after its first reported measurements and calculations for phonons in suspended nanostructures, reconciling experiments and theory remains elusive. Our massively parallel calculations of phonon transport in micrometer-sized three-dimensional structures suggest that part of the disagreement between theory and experiment stems from the inadequacy of macroscopic concepts to analyze the data. The computed local temperature distribution in the wave ballistic nonequilibrium regime shows that the spatial placement and dimensions of thermometers, heaters, and supporting microbeams in the suspended structures can noticeably affect the thermal conductance's measured values. In addition, diffusive transport assumptions made in the data analysis may result in measured values that considerably differ from the actual thermal conductance of the structure. These results urge for experimental validation of the suitability of diffusive transport assumptions in measuring devices operating at sub-kelvin temperatures.

摘要

热导量子是量子输运理论中的一个基本量。然而,在首次报道对悬浮纳米结构中的声子进行测量和计算二十年后,使实验与理论相协调仍然难以实现。我们对微米级三维结构中的声子输运进行的大规模并行计算表明,理论与实验之间的部分分歧源于宏观概念在分析数据时的不足。在波动弹道非平衡状态下计算得到的局部温度分布表明,悬浮结构中温度计、加热器和支撑微梁的空间位置及尺寸会显著影响热导的测量值。此外,数据分析中所做的扩散输运假设可能导致测量值与结构的实际热导有很大差异。这些结果促使人们对在亚开尔文温度下运行的测量设备中扩散输运假设的适用性进行实验验证。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/d7533a2d095d/sciadv.adi7439-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/bc89393fc5a9/sciadv.adi7439-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/53eb633b5916/sciadv.adi7439-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/13d59b2b5cf0/sciadv.adi7439-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/206fca9b1593/sciadv.adi7439-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/4ccbd3fac1a7/sciadv.adi7439-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/1864b7ba4db1/sciadv.adi7439-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/d7533a2d095d/sciadv.adi7439-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/bc89393fc5a9/sciadv.adi7439-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/53eb633b5916/sciadv.adi7439-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/13d59b2b5cf0/sciadv.adi7439-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/206fca9b1593/sciadv.adi7439-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/4ccbd3fac1a7/sciadv.adi7439-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/1864b7ba4db1/sciadv.adi7439-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3884/11090371/d7533a2d095d/sciadv.adi7439-f7.jpg

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本文引用的文献

1
Heat conduction measurements in ballistic 1D phonon waveguides indicate breakdown of the thermal conductance quantization.在弹道一维声子波导中的热传导测量表明,热导量化的崩溃。
Nat Commun. 2018 Oct 16;9(1):4287. doi: 10.1038/s41467-018-06791-0.
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