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少层ReS₂中与温度相关的传导和光响应

Temperature-Dependent Conduction and Photoresponse in Few-Layer ReS.

作者信息

Intonti Kimberly, Faella Enver, Kumar Arun, Viscardi Loredana, Giubileo Filippo, Martucciello Nadia, Lam Hoi Tung, Anastasiou Konstantinos, Craciun Monica, Russo Saverio, Di Bartolomeo Antonio

机构信息

Department of Physics "E.R. Caianiello", University of Salerno, Fisciano 84084, Salerno, Italy.

CNR-SPIN, Fisciano 84084, Salerno, Italy.

出版信息

ACS Appl Mater Interfaces. 2023 Nov 1;15(43):50302-50311. doi: 10.1021/acsami.3c12973. Epub 2023 Oct 20.

Abstract

The electrical behavior and the photoresponse of rhenium disulfide field-effect transistors (FETs) have been widely studied; however, only a few works have investigated the photocurrent as a function of temperature. In this paper, we perform the electrical characterization of few-layer ReS-based FETs with Cr-Au contacts over a wide temperature range. We exploit the temperature-dependent transfer and output characteristics to estimate the effective Schottky barrier at the Cr-Au/ReS interface and to investigate the temperature behavior of parameters, such as the threshold voltage, carrier concentration, mobility, and subthreshold swing. Through time-resolved photocurrent measurements, we show that the photocurrent increases with temperature and exhibits a linear dependence on the incident light power at both low and room temperatures and a longer rise/decay time at higher temperatures. We surmise that the photocurrent is affected by the photobolometric effect and light-induced desorption of adsorbates which are facilitated by the high temperature and the low pressure.

摘要

二硫化铼场效应晶体管(FET)的电学行为和光响应已得到广泛研究;然而,仅有少数研究探讨了光电流与温度的关系。在本文中,我们对具有Cr-Au接触的几层ReS基FET在很宽的温度范围内进行了电学表征。我们利用与温度相关的转移和输出特性来估计Cr-Au/ReS界面处的有效肖特基势垒,并研究诸如阈值电压、载流子浓度、迁移率和亚阈值摆幅等参数的温度行为。通过时间分辨光电流测量,我们发现光电流随温度升高而增加,并且在低温和室温下对入射光功率均呈现线性依赖关系,而在较高温度下具有更长的上升/衰减时间。我们推测,光电流受到光热效应以及高温和低压促进的吸附质光致解吸的影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/83e3/10623565/8071b4684160/am3c12973_0001.jpg

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