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用于皮秒时间分辨共振软X射线散射和光谱学的多功能桌面装置。

Versatile tabletop setup for picosecond time-resolved resonant soft-x-ray scattering and spectroscopy.

作者信息

Borchert Martin, Braenzel Julia, Gnewkow Richard, Lunin Leonid, Sidiropoulos Themistoklis, Tümmler Johannes, Will Ingo, Noll Tino, Reichel Oliver, Rohloff Dirk, Erko Alexei, Krist Thomas, von Korff Schmising Clemens, Pfau Bastian, Eisebitt Stefan, Stiel Holger, Schick Daniel

机构信息

Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie, 12489 Berlin, Germany.

Helmholtz-Zentrum Berlin, 12489 Berlin, Germany.

出版信息

Rev Sci Instrum. 2023 Jun 1;94(6). doi: 10.1063/5.0151613.

Abstract

We present a laser-driven, bright, and broadband (50 to 1500 eV) soft-x-ray plasma source with <10 ps pulse duration. This source is employed in two complementary, laboratory-scale beamlines for time-resolved, magnetic resonant scattering and spectroscopy, as well as near-edge x-ray absorption fine-structure (NEXAFS) spectroscopy. In both beamlines, dedicated reflection zone plates (RZPs) are used as single optical elements to capture, disperse, and focus the soft x rays, reaching resolving powers up to E/ΔE > 1000, with hybrid RZPs at the NEXAFS beamline retaining a consistent E/ΔE > 500 throughout the full spectral range, allowing for time-efficient data acquisition. We demonstrate the versatility and performance of our setup by a selection of soft-x-ray spectroscopy and scattering experiments, which so far have not been possible on a laboratory scale. Excellent data quality, combined with experimental flexibility, renders our approach a true alternative to large-scale facilities, such as synchrotron-radiation sources and free-electron lasers.

摘要

我们展示了一种由激光驱动的、明亮且宽带(50至1500电子伏特)的软X射线等离子体源,其脉冲持续时间小于10皮秒。该源用于两条互补的实验室规模光束线,用于时间分辨磁共振散射和光谱学以及近边X射线吸收精细结构(NEXAFS)光谱学。在这两条光束线中,专用反射波带片(RZPs)被用作单一光学元件来捕获、色散和聚焦软X射线,分辨率高达E/ΔE > 1000,NEXAFS光束线的混合RZPs在整个光谱范围内保持一致的E/ΔE > 500,从而实现高效的数据采集。我们通过一系列软X射线光谱学和散射实验展示了我们装置的多功能性和性能,这些实验迄今为止在实验室规模上是无法实现的。出色的数据质量与实验灵活性相结合,使我们的方法成为同步辐射源和自由电子激光等大型设施的真正替代方案。

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