School of Chemistry, Food Biosciences and Pharmacy, University of Reading, Whiteknights, Reading RG6 6AD, United Kingdom.
Departamento de Biofísica, Universidade Federal de São Paulo, São Paulo 04023-062, Brazil.
Biomacromolecules. 2023 Nov 13;24(11):5403-5413. doi: 10.1021/acs.biomac.3c00860. Epub 2023 Nov 1.
There has been considerable interest in peptides in which the Fmoc (9-fluorenylmethoxycarbonyl) protecting group is retained at the N-terminus, since this bulky aromatic group can drive self-assembly, and Fmoc-peptides are biocompatible and have applications in cell culture biomaterials. Recently, analogues of new amino acids with 2,7-disulfo-9-fluorenylmethoxycarbonyl (Smoc) protecting groups have been developed for water-based peptide synthesis. Here, we report on the self-assembly and biocompatibility of Smoc-Ala, Smoc-Phe and Smoc-Arg as examples of Smoc conjugates to aliphatic, aromatic, and charged amino acids, respectively. Self-assembly occurs at concentrations above the critical aggregation concentration (CAC). Cryo-TEM imaging and SAXS reveal the presence of nanosheet, nanoribbon or nanotube structures, and spectroscopic methods (ThT fluorescence circular dichroism and FTIR) show the presence of β-sheet secondary structure, although Smoc-Ala solutions contain significant unaggregated monomer content. Smoc shows self-fluorescence, which was used to determine CAC values of the Smoc-amino acids from fluorescence assays. Smoc fluorescence was also exploited in confocal microscopy imaging with fibroblast cells, which revealed its uptake into the cytoplasm. The biocompatibility of these Smoc-amino acids was found to be excellent with zero cytotoxicity (in fact increased metabolism) to fibroblasts at low concentration.
人们对 N 端保留 Fmoc(9-芴甲氧羰基)保护基的肽类化合物产生了浓厚的兴趣,因为这种庞大的芳基基团可以驱动自组装,并且 Fmoc-肽具有生物相容性,并在细胞培养生物材料中有应用。最近,开发了带有 2,7-二磺酸-9-芴甲氧羰基(Smoc)保护基的新型氨基酸类似物,用于水相肽合成。在这里,我们报告了 Smoc-Ala、Smoc-Phe 和 Smoc-Arg 作为 Smoc 缀合物的实例,分别为脂肪族、芳香族和带电荷的氨基酸的自组装和生物相容性。自组装在超过临界聚集浓度 (CAC) 的浓度下发生。冷冻 TEM 成像和 SAXS 显示存在纳米片、纳米带或纳米管结构,光谱方法(ThT 荧光圆二色性和 FTIR)显示存在β-折叠二级结构,尽管 Smoc-Ala 溶液含有大量未聚集的单体。Smoc 具有自荧光,可用于从荧光测定中确定 Smoc-氨基酸的 CAC 值。Smoc 荧光还被用于成纤维细胞的共聚焦显微镜成像,揭示了其进入细胞质的情况。这些 Smoc-氨基酸的生物相容性非常好,在低浓度下对成纤维细胞没有细胞毒性(实际上增加了代谢)。