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快速氖原子在LiF表面的弹性和非弹性衍射

Elastic and inelastic diffraction of fast neon atoms on a LiF surface.

作者信息

Debiossac Maxime, Pan Peng, Roncin Philippe

机构信息

Université Paris-Saclay, CNRS, Institut des Sciences Moléculaires d'Orsay (ISMO), 91405 Orsay, France.

出版信息

Phys Chem Chem Phys. 2023 Nov 22;25(45):30966-30974. doi: 10.1039/d3cp04034h.

Abstract

Grazing incidence fast atom diffraction has mainly been investigated with helium atoms, considered as the best possible choice for surface analysis. This article presents experimental diffraction profiles recorded with neon projectile, between 300 eV and 4 keV kinetic energy with incidence angles between 0.3 and 1.5° along three different directions of a LiF(001) crystal surface. These correspond to perpendicular energy ranging from a few meV up to almost 1 eV. A careful analysis of the scattering profile allows us to extract the diffracted intensities even when inelastic effects become so large that most quantum signatures have disappeared. The relevance of this approach is discussed in terms of surface topology.

摘要

掠入射快原子衍射主要是用氦原子进行研究的,氦原子被认为是表面分析的最佳选择。本文展示了用氖离子在300电子伏特至4千电子伏特的动能下,沿着LiF(001)晶体表面的三个不同方向,以0.3至1.5°的入射角记录的实验衍射轮廓。这些对应于从几毫电子伏特到几乎1电子伏特的垂直能量。对散射轮廓的仔细分析使我们能够提取衍射强度,即使非弹性效应变得如此之大,以至于大多数量子特征都消失了。本文从表面拓扑结构的角度讨论了这种方法的相关性。

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