Hou Lu, Zhu Yuan-Yuan, Liu Bing, Li Jian-Jun
China National Environmental Monitoring Centre, Beijing 100012, China.
Huan Jing Ke Xue. 2023 Nov 8;44(11):5899-5914. doi: 10.13227/j.hjkx.202211270.
From January 31 to February 20, 2015 to 2022, the spatio-temporal characteristics of the PM pollution evolution of 44 cities in the Beijing-Tianjin-Hebei Region and its surrounding areas were analyzed. The contribution of simultaneous meteorology, coordinated emission reduction, and cross-regional transmission to PM concentration and chemical component changes were quantified, respectively, with the aim to provide scientific reference for regional air quality joint prevention and control under adverse meteorological conditions. The results showed that the mean value of PM concentration of 44 cities in 2022 was the lowest(46 μg·m) without heavy pollution in the same period of the lunar calendar since 2015, whereas the proportion of days with good air quality was the highest(83.3%). PM pollution was more serious in the southern region than that in the northern region, and the high values were mainly concentrated along the Taihang Mountains and Yanshan transmission channel cities. In 2016, under the unregulated emission of fireworks in the Spring Festival, the proportion of unpolluted days was 93.5%, which means that the strong atmospheric diffusion ability was crucial to improve air quality. In 2022, the static weather index(SWI) increased by 2.1 compared with that in 2021, indicating unfavorable atmospheric diffusion capacity. The average and peak values of PM decreased by 14 μg·m and 76 μg·m, respectively. The reduction in PM concentration in Beijing owing to emission reduction measures increased by 96% compared with that before one month. Under the adverse atmospheric background in the Shanxi-Shandong-Henan Region, which contributed to the increase in PM concentration, the peak value of PM concentration decreased by 87 μg·m, indicating that the peak clipping effect of regional collaborative pollution emission reduction was significant. From 2019 to 2022, the concentration of PM chemical components decreased yearly with narrowed spatial differences, and the high value was concentrated in the central and southern regions. The descending order of PM secondary component concentration decrease was as follows:organic matter(21.9%)>sulfate(20%)>ammonium salt(16.7%)>nitrate(9.7%). The proportion of nitrate in PM increased yearly to 30.1%, indicating that the contribution of traffic pollution was relatively prominent. In 2022, the SNA concentration in the Shanxi-Shandong-Henan Region increased. Pollution from external sources accounted for the main contribution in the Beijing-Tianjin-Hebei Region(>50%). Liaoning Province contributed significantly to the PM concentration in cities along the Bohai(>10%), and nitrate and sulfate were easy to transport over long distances. It is necessary to strengthen the coordinated control of precursors of secondary chemical components SO, NO, and NH.
对2015年至2022年1月31日至2月20日京津冀地区及周边44个城市PM污染演变的时空特征进行了分析。分别量化了同期气象、协同减排和跨区域传输对PM浓度和化学成分变化的贡献,旨在为不利气象条件下区域空气质量联防联控提供科学参考。结果表明,2022年44个城市PM浓度均值为2015年以来同期最低(46μg·m),且无重度污染,空气质量优良天数比例最高(83.3%)。南部地区PM污染比北部地区更严重,高值主要集中在太行山和燕山传输通道沿线城市。2016年春节烟花燃放未管控,未污染天数比例为93.5%,这表明强大气扩散能力对改善空气质量至关重要。2022年,静稳天气指数(SWI)较2021年上升2.1,表明大气扩散能力不利。PM均值和峰值分别下降了14μg·m和76μg·m。北京因减排措施导致的PM浓度下降较前一个月增加了96%。在山西-山东-河南地区不利大气背景导致PM浓度上升的情况下,PM浓度峰值下降了87μg·m,表明区域协同污染减排削峰效果显著。2019年至2022年,PM化学成分浓度逐年下降,空间差异缩小,高值集中在中南部地区。PM二次成分浓度下降幅度由大到小依次为:有机物(21.9%)>硫酸盐(20%)>铵盐(16.7%)>硝酸盐(9.7%)。PM中硝酸盐比例逐年上升至30.1%,表明交通污染贡献相对突出。2022年,山西-山东-河南地区SNA浓度上升。京津冀地区外来源污染贡献占主导(>50%)。辽宁省对渤海沿岸城市PM浓度贡献显著(>10%),硝酸盐和硫酸盐易于远距离传输。有必要加强对二次化学成分SO、NO和NH前体物的协同控制。