Ji Jianyu, Qian Shizhi, Parker Armani Marie, Zhang Xiaoyu
Department of Mechanical and Aerospace Engineering, Old Dominion University, Norfolk, VA 23529, USA.
Micromachines (Basel). 2023 Nov 8;14(11):2077. doi: 10.3390/mi14112077.
Electroosmotic flow (EOF) is of utmost significance due to its numerous practical uses in controlling flow at micro/nanoscales. In the present study, the time-periodic EOF of a viscoelastic fluid is statistically analyzed using a short 10:1 constriction microfluidic channel joining two reservoirs on either side. The flow is modeled using the Oldroyd-B (OB) model and the Poisson-Boltzmann model. The EOF of a highly concentrated polyacrylamide (PAA) aqueous solution is investigated under the combined effects of an alternating current (AC) electric field and a direct current (DC) electric field. Power-law degradation is visible in the energy spectra of the velocity fluctuations over a wide frequency range, pointing to the presence of elastic instabilities in the EOF. The energy-spectra curves of the velocity fluctuations under a DC electric field exhibit peaks primarily beneath 20 Hz, with the greatest peak being observed close to 6 Hz. When under both DC and AC electric fields, the energy spectra of the velocity fluctuations exhibit a peak at the same frequency as the AC electric field, and the highest peak is obtained when the frequency of the AC electric field is near 6 Hz. Additionally, the frequency of the AC electric field affects how quickly the viscoelastic EOF flows. Higher flow rates are obtained at relatively low frequencies compared to under the DC electric field, and the greatest flow rate is found close to 6 Hz. But as the frequency rises further, the flow rate falls. The flow rate falls to a level below the DC electric field when the frequency is sufficiently high.
电渗流(EOF)因其在微纳尺度下控制流体流动方面的众多实际应用而具有极其重要的意义。在本研究中,使用一个短的10:1收缩微流控通道对粘弹性流体的周期性电渗流进行了统计分析,该通道连接两侧的两个储液器。采用Oldroyd - B(OB)模型和泊松 - 玻尔兹曼模型对流动进行建模。研究了在交流(AC)电场和直流(DC)电场联合作用下高浓度聚丙烯酰胺(PAA)水溶液的电渗流。在很宽的频率范围内,速度波动的能谱中可见幂律衰减,这表明电渗流中存在弹性不稳定性。直流电场下速度波动的能谱曲线主要在20Hz以下出现峰值,最大峰值出现在接近6Hz处。当同时施加直流和交流电场时,速度波动的能谱在与交流电场相同的频率处出现峰值,且当交流电场频率接近6Hz时获得最高峰值。此外,交流电场的频率会影响粘弹性电渗流的流动速度。与直流电场相比,在相对较低的频率下可获得更高的流速,最大流速出现在接近6Hz处。但随着频率进一步升高,流速下降。当频率足够高时,流速降至直流电场以下的水平。