Tutunnikov Ilia, Chuang Chern, Cao Jianshu
Department of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, United States.
Department of Chemistry and Biochemistry, University of Nevada, 4505 S Maryland Pkwy, Las Vegas, Nevada 89154, United States.
J Phys Chem Lett. 2023 Dec 28;14(51):11632-11639. doi: 10.1021/acs.jpclett.3c03047. Epub 2023 Dec 15.
Quantum lattices are pivotal in the burgeoning fields of quantum materials and information science. Novel experimental techniques allow the preparation and monitoring of wave packet dynamics on quantum lattices with high spatiotemporal resolution. We present an analytical study of wave packet diffusivity and diffusion length on tight-binding quantum lattices subject to stochastic noise. Our analysis reveals the crucial role of spatial coherence and predicts a set of novel phenomena: (1) noise can enhance the transient diffusivity and diffusion length of spatially extended initial states; (2) standing or traveling initial states, with large momentum, spread faster than a localized initial state and exhibit a noise-induced peak in the transient diffusivity; (3) the differences in the diffusivity or diffusion length of extended and localized initial states have a universal dependence on initial width. These predictions suggest the possibility of controlling the wave packet dynamics by spatial manipulations, which will have implications for materials science and quantum technologies.
量子晶格在量子材料和信息科学的新兴领域中起着关键作用。新颖的实验技术能够以高时空分辨率制备和监测量子晶格上的波包动力学。我们对受随机噪声影响的紧束缚量子晶格上的波包扩散率和扩散长度进行了分析研究。我们的分析揭示了空间相干性的关键作用,并预测了一系列新现象:(1)噪声可以增强空间扩展初始态的瞬态扩散率和扩散长度;(2)具有大动量的驻波或行波初始态比局域化初始态传播得更快,并且在瞬态扩散率中表现出噪声诱导的峰值;(3)扩展和局域化初始态的扩散率或扩散长度差异对初始宽度具有普遍依赖性。这些预测表明通过空间操纵来控制波包动力学的可能性,这将对材料科学和量子技术产生影响。