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基于源的土壤重金属污染健康风险评估:以中国中部鄂东南某多金属矿区为例。

Source-based health risk assessment of heavy metal contamination in soil: a case study from a polymetallic mining region in Southeastern Hubei, Central China.

机构信息

School of Environmental Science and Engineering, Hubei Polytechnic University, Huangshi, 435003, China.

Hubei Key Laboratory of Mine Environmental Pollution Control and Remediation, Hubei Polytechnic University, Huangshi, 435003, China.

出版信息

Environ Geochem Health. 2023 Dec 26;46(1):12. doi: 10.1007/s10653-023-01804-4.

Abstract

To conduct a precise health risk assessment of heavy metals (HMs) in soil, it is imperative to ascertain the primary sources of potential health risks. In this study, we conducted comprehensive measurements of HMs, specifically focusing on the accumulation of Cu, Cd, Sb, Zn, and Pb in local soil, which may pose threats to environmental quality. To achieve our objective, we employed a method that combines positive matrix factorization with a health risk assessment model to quantify the health risks associated with specific sources. The results obtained from the geo-accumulation index indicate that the majority of HMs found in the local soil are influenced by anthropogenic activities. Among these sources, local industrial-related activities contributed the largest proportion of HMs to the soil at 34.7%, followed by natural sources at 28.7%, mining and metallurgy-related activities at 28.2%, and traffic-related activities at 8.40%. Although the non-carcinogenic and carcinogenic risks associated with individual HMs were found to be below safety thresholds, the cumulative health risks stemming from total HMs exceeded safety limits for children. Moreover, the unacceptable health risks for children originating from industrial-related activities, natural sources, and mining and metallurgy-related activities were primarily concentrated in proximity to mining sites and industrial areas within the local region. This investigation furnishes valuable insights that can aid governmental authorities in formulating precise control policies to mitigate health threats posed by soils in polymetallic mining areas.

摘要

为了对土壤中的重金属(HMs)进行精确的健康风险评估,确定潜在健康风险的主要来源至关重要。在这项研究中,我们对 HMs 进行了全面测量,特别是关注 Cu、Cd、Sb、Zn 和 Pb 在当地土壤中的积累,这些元素可能对环境质量构成威胁。为了实现我们的目标,我们采用了一种将正定矩阵分解与健康风险评估模型相结合的方法,以量化与特定来源相关的健康风险。地积累指数的结果表明,当地土壤中发现的大多数 HMs 受到人为活动的影响。在这些来源中,本地工业相关活动对土壤中 HMs 的贡献最大,占 34.7%,其次是自然来源,占 28.7%,采矿和冶金相关活动占 28.2%,交通相关活动占 8.40%。尽管个别 HMs 的非致癌和致癌风险被发现低于安全阈值,但总 HMs 对儿童的累积健康风险超过了安全限制。此外,儿童的不可接受健康风险主要来自工业相关活动、自然来源和采矿及冶金相关活动,这些风险主要集中在当地矿区和工业区附近。这项调查提供了有价值的见解,可以帮助政府当局制定精确的控制政策,以减轻多金属矿区土壤带来的健康威胁。

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