Nuclear Technology Laboratory, Department of Electrical and Computer Engineering, Aristotle University of Thessaloniki, Thessaloniki GR-54124, Greece.
German Aerospace Center (DLR), Institute for the Protection of Terrestrial Infrastructure, Sankt Augustin 53757, Germany.
Radiat Prot Dosimetry. 2024 Mar 20;200(4):339-354. doi: 10.1093/rpd/ncad309.
This study focused on assessing the risk from the exposure to radon contained in domestic water for a significant part (~20%) of the Greek population. Also, the variation of radon in domestic water was monitored from 2017 to 2023 in certain villages that showed relatively high radon levels and relied on boreholes for their water supply. The radon in domestic water activity concentrations measured in the investigated Greek places ranged from lower than the minimum detection limit (2 Bq L-1) levels up to 187 Bq L-1 with an average value of 9.1 Bq L-1. Overall, higher radon in domestic water activity concentrations were observed in places supplied from boreholes located inside granitic and metamorphic rock areas. Only one out of the 487 examined places, which accounts for 0.015% of the examined Greek population, showed an average radon-in-water activity concentration higher than the parametric value of 100 Bq L-1 adopted by Greece following the EURATOM Directive (2013/51/EURATOM). Therefore, radon-in-water does not pose a health concern (risk) for the investigated Greek population. The total (inhalation and ingestion) annual effective doses to adults, corresponding to the measured radon-in-water activity concentrations, ranged from nearly 0 to 1.20 mSv y-1 with an average value of 0.059 mSv y-1, while for children, they ranged from almost 0 to 1.26 mSv y-1 with an average value of 0.061 mSv y-1. Regarding the variation of radon in domestic water monitoring, places supplied with water from one borehole showed no significant fluctuations from their average radon-in-water activity concentration, with standard deviations of ~20% at a coverage factor of k = 1. Even though some places supplied from three to four boreholes showed no significant fluctuations (standard deviation <= 30% at k = 1) from their average radon level, special attention is needed for places supplied from many boreholes when one measurement over the year is to be performed for the annual effective dose assessment. This is because the prevailing during-year borehole combination may not exist on the measurement day, resulting in an underestimated or overestimated dose assessment. Radon removal from domestic water supplies in the Arnea village (due to elevated radon-in-water activity concentrations) did not affect the inhalation risk for the residents of an examined house in Arnea. However, radon removal from the water supply was essential to reduce the ingestion risk for the house occupants. There is a possibility of radiation overexposure (>20 mSv y-1) for the workers in a thermal spa on Ikaria Island, and further investigation needs to be conducted with extended measurement periods.
本研究重点评估了希腊约 20%人口家中饮用水中所含氡的暴露风险。此外,在某些村庄监测了 2017 年至 2023 年期间饮用水中氡的变化情况,这些村庄的氡水平相对较高,且依赖水井供水。在研究的希腊地区,测量的饮用水氡活度浓度范围从低于检测下限(2 Bq L-1)水平到 187 Bq L-1,平均值为 9.1 Bq L-1。总体而言,来自花岗岩和变质岩地区内钻孔的供水地区的饮用水氡活度浓度较高。在所检查的 487 个地方中,只有一个地方(占检查的希腊人口的 0.015%)的平均氡水活度浓度高于希腊根据 EURATOM 指令(2013/51/EURATOM)采用的 100 Bq L-1 参数值。因此,饮用水中的氡不会对所研究的希腊人口构成健康(风险)威胁。与测量的饮用水氡活度浓度相对应的成年人的总(吸入和摄入)年有效剂量从几乎为零到 1.20 mSv y-1,平均值为 0.059 mSv y-1,而对于儿童,他们的剂量范围从几乎为零到 1.26 mSv y-1,平均值为 0.061 mSv y-1。关于饮用水中氡的监测变化,来自一个钻孔供水的地方的氡活度浓度没有明显波动,标准偏差约为 20%,置信因子 k=1。尽管来自三个到四个钻孔的一些地方的平均氡水平没有明显波动(k=1 时标准偏差<=30%),但对于使用多个钻孔供水的地方,需要特别注意,因为在一年中仅进行一次测量以进行年有效剂量评估。这是因为一年中存在的钻孔组合在测量日可能不存在,导致剂量评估低估或高估。由于饮用水中氡的活度浓度较高,Arnea 村的饮用水供应中的氡去除并未影响 Arnea 受检房屋居民的吸入风险。然而,去除水中的氡对于房屋居住者的摄入风险至关重要。伊卡里亚岛上的一个温泉浴场的工人可能存在辐射过度暴露(>20 mSv y-1)的风险,需要进一步延长测量周期进行调查。