Liu Mingxiu, Wei Jingxuan, Qi Liujian, An Junru, Liu Xingsi, Li Yahui, Shi Zhiming, Li Dabing, Novoselov Kostya S, Qiu Cheng-Wei, Li Shaojuan
State Key Laboratory of Luminescence and Applications, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Jilin, 130033, Changchun, PR China.
University of Chinese Academy of Sciences (UCAS), 100049, Beijing, PR China.
Nat Commun. 2024 Jan 2;15(1):141. doi: 10.1038/s41467-023-44482-7.
Photogating effect is the dominant mechanism of most high-responsivity two-dimensional (2D) material photodetectors. However, the ultrahigh responsivities in those devices are intrinsically at the cost of very slow response speed. In this work, we report a WSe/TaNiSe heterostructure detector whose photodetection gain and response speed can be enhanced simultaneously, overcoming the trade-off between responsivity and speed. We reveal that photogating-assisted tunneling synergistically allows photocarrier multiplication and carrier acceleration through tunneling under an electrical field. The photogating effect in our device features low-power consumption (in the order of nW) and shows a dependence on the polarization states of incident light, which can be further tuned by source-drain voltages, allowing for wavelength discrimination with just a two-electrode planar structure. Our findings offer more opportunities for the long-sought next-generation photodetectors with high responsivity, fast speed, polarization detection, and multi-color sensing, simultaneously.
光门控效应是大多数高响应性二维材料光电探测器的主要机制。然而,这些器件中的超高响应度本质上是以非常慢的响应速度为代价的。在这项工作中,我们报道了一种WSe/TaNiSe异质结构探测器,其光电探测增益和响应速度可以同时提高,克服了响应度和速度之间的权衡。我们揭示了光门控辅助隧穿协同作用使得光载流子倍增以及载流子在电场作用下通过隧穿加速。我们器件中的光门控效应具有低功耗(纳瓦级)的特点,并且表现出对入射光偏振态的依赖性,这可以通过源漏电压进一步调节,仅采用两电极平面结构就能实现波长辨别。我们的发现为长期以来寻求的同时具有高响应度、快速速度、偏振检测和多色传感功能的下一代光电探测器提供了更多机会。