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窟野河流域沉积物中多环芳烃的分布特征、来源分析及生态风险评价:一个典型的能源化工区河流。

Distribution characteristics, source analysis and risk assessment of polycyclic aromatic hydrocarbons in sediments of Kuye River: a river in a typical energy and chemical industry zone.

机构信息

School of Environmental and Municipal Engineering, Xi'an University of Architecture and Technology, Yan Ta Road. No.13, Xi'an, 710055, China.

Key Lab of Northwest Water Resource, Environment and Ecology, Ministry of Education, Xi'an University of Architecture and Technology, Xi'an, 710055, China.

出版信息

Environ Geochem Health. 2024 Feb 17;46(3):89. doi: 10.1007/s10653-023-01802-6.

Abstract

This study systematically analyzed the distribution characteristics, sources, and ecological risk of polycyclic aromatic hydrocarbons (PAHs) in Kuye River sediments, located in an energy and chemical industry base in northern Shaanxi, China. The results that revealed the concentrations of 16 PAHs in the sediment ranged from 1090.04 to 32,175.68 ng∙g dw, with the four-ring PAHs accounting for the highest proportion. Positive matrix factorization analysis (PMF) revealed the main sources of PAHs as incomplete fossil fuel combustion, biomass combustion, and traffic emissions. The total toxic equivalent concentration of BaP, risk quotient, and lifetime carcinogenic risk of PAHs suggested moderate to high contamination of PAHs in the area. The higher incremental lifetime carcinogenic risk (ILCR) indicated that PAH ingestion was the primary route of impact on public health, with children potentially being more susceptible to PAH exposure. This study can provide valuable theoretical support for implementing pollution prevention measures and ecological restoration strategies for rivers in energy and chemical industry areas.

摘要

本研究系统分析了位于中国陕北能源化工基地窟野河沉积物中多环芳烃(PAHs)的分布特征、来源和生态风险。结果表明,沉积物中 16 种 PAHs 的浓度范围为 1090.04 至 32175.68ng·g dw,四环 PAHs 所占比例最高。正定矩阵因子分析(PMF)揭示了 PAHs 的主要来源为不完全化石燃料燃烧、生物质燃烧和交通排放。BaP 的总毒性当量浓度、风险商和 PAHs 的终生致癌风险表明该地区 PAHs 污染处于中等偏高水平。较高的增量终生致癌风险(ILCR)表明,PAH 的摄入是影响公众健康的主要途径,儿童可能更容易受到 PAH 的暴露。本研究可为能源化工区河流实施污染防治措施和生态修复策略提供有价值的理论支持。

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