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中国东部某特大城市城市道路灰尘中微塑料的时空分布及特征

Spatiotemporal occurrence and characteristics of microplastics in the urban road dust in a megacity, eastern China.

作者信息

Fan Yifan, Zheng Jinglan, Xu Wanlu, Zhang Qiji, Chen Nianhao, Wang Hui, Qian Xin, Wang Guoqiang

机构信息

State Key Laboratory of Pollution Control and Resources Reuse, School of Environment, Nanjing University, Nanjing 210023, China.

State Key Laboratory of Pollution Control and Resources Reuse, School of Environment, Nanjing University, Nanjing 210023, China; SinoCarbon Innovation & Investment (SCII) Co., Ltd., Beijing 100000, China.

出版信息

J Hazard Mater. 2024 Apr 15;468:133733. doi: 10.1016/j.jhazmat.2024.133733. Epub 2024 Feb 8.

Abstract

The pervasive issue of microplastics pollution has garnered public attention, yet urban residents remain unaware of the threat within their living spaces. Urban road dust, as primary reservoirs for environmental microplastics, offers an insightful perspective into their occurrence and characteristics. This study investigated microplastics in the urban road dust in Nanjing, a megacity in eastern China, to reveal their spatiotemporal pattern. The abundance of microplastics in the road dust measured 143.3 ± 40.8 particles/m, with predominant fragments and suspected tire wear particles, particularly those below 100 µm. Significant spatial variations were observed across urban functional zones (P < 0.05), with commercial and heavy industrial areas experiencing the highest microplastic pollution (up to 223.5 particles/m). Infrared spectroscopy analysis identified 29 polymer types, with polystyrene (PS), polyamide (PA), and polyvinylidene difluoride (PVDF) prevailing. Light industrial zones exhibited slight contamination (mean = 93.4 particles/m) but with diverse polymer components (24 types). Redundancy analysis and variation partitioning revealed that urban functional zoning, 7-day accumulated precipitation, and monthly PM primarily influenced the occurrence and characteristics of microplastics in urban road dust (P = 0.001). This study deepened our understanding of microplastics pollution in urban environments, providing novel insights for effective urban environmental management and improvement.

摘要

微塑料污染这一普遍问题已引起公众关注,但城市居民仍未意识到其居住空间内的威胁。城市道路灰尘作为环境微塑料的主要储存库,为了解其存在情况和特征提供了一个有洞察力的视角。本研究调查了中国东部大城市南京城市道路灰尘中的微塑料,以揭示其时空格局。道路灰尘中微塑料的丰度为143.3±40.8颗粒/米,主要为碎片和疑似轮胎磨损颗粒,尤其是那些小于100微米的颗粒。在城市功能区观察到显著的空间差异(P<0.05),商业区和重工业区的微塑料污染最高(高达223.5颗粒/米)。红外光谱分析确定了29种聚合物类型,其中聚苯乙烯(PS)、聚酰胺(PA)和聚偏二氟乙烯(PVDF)占主导地位。轻工业区污染较轻(平均=93.4颗粒/米),但聚合物成分多样(24种)。冗余分析和变异分解表明,城市功能分区、7天累计降水量和月均颗粒物主要影响城市道路灰尘中微塑料的存在情况和特征(P=0.001)。本研究加深了我们对城市环境中微塑料污染的理解,为有效的城市环境管理和改善提供了新的见解。

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