Yao Fang, Dong Kailian, Ke Weijun, Fang Guojia
Key Lab of Artificial Micro- and Nano-Structures of Ministry of Education of China, School of Physics and Technology, Wuhan University, Wuhan 430072, People's Republic of China.
School of Electronic and Electrical Engineering, Wuhan Textile University, Wuhan 430200, People's Republic of China.
ACS Nano. 2024 Feb 27;18(8):6095-6110. doi: 10.1021/acsnano.3c10116. Epub 2024 Feb 19.
Halide perovskites have emerged as highly promising materials for ionizing radiation detection due to their exceptional characteristics, including a large mobility-lifetime product, strong stopping power, tunable band gap, and cost-effective crystal growth via solution processes. Semiconductor-type X-ray detectors employing various micro/nano perovskite materials have shown impressive progress in achieving heightened sensitivity and lower detection limits. Here, we present a comprehensive review of the applications of micro/nano perovskite materials for direct type X-ray detection, with a focus on the requirements for micro/nano crystal assembly and device properties in advanced X-ray detectors. We explore diverse processing techniques and optoelectronic considerations applied to perovskite X-ray detectors. Additionally, this review highlights the challenges and promising opportunities for perovskite X-ray detector arrays in real-world applications, potentially necessitating further research efforts.
卤化物钙钛矿因其优异的特性,包括大的迁移率-寿命乘积、强阻止本领、可调节的带隙以及通过溶液法实现具有成本效益的晶体生长,已成为极具前景的电离辐射探测材料。采用各种微/纳米钙钛矿材料的半导体型X射线探测器在提高灵敏度和降低探测限方面已取得了令人瞩目的进展。在此,我们全面综述了微/纳米钙钛矿材料在直接型X射线探测中的应用,重点关注先进X射线探测器中微/纳米晶体组装的要求和器件性能。我们探讨了应用于钙钛矿X射线探测器的各种加工技术和光电考量因素。此外,本综述强调了钙钛矿X射线探测器阵列在实际应用中的挑战和潜在的机遇,这可能需要进一步的研究工作。