College of Civil Engineering and Architecture, Zhejiang University, 866 Yuhangtang Road, Hangzhou, 310027, China.
Center for Balance Architecture, Zhejiang University, 148 Tianmushan Road, Hanghzou, 310007, China.
Environ Sci Pollut Res Int. 2024 Mar;31(14):21765-21780. doi: 10.1007/s11356-024-32554-0. Epub 2024 Feb 23.
In recent years, heavy metal contamination of soils has become a major concern in China due to the potential risks involved. To assess environmental pollution and human health risks in a typical heavy metal polluted site in Jiangxi Province, a thorough evaluation of the distribution, pollution levels, and sources of heavy metals in soils of the Yangmeijiang River watershed was conducted in this study. Positive matrix factorization and Monte Carlo simulation were used to evaluate the ecological and human health risks of heavy metals. The research findings indicate that heavy metal pollution was the most severe at the depth of 20-40 cm in soils, with local heavy metal pollution resulting from mining and sewage irrigation. The high-risk area accounted for 91.11% of the total area. However, the pollution level decreased with time due to sampling effects, rainfall, and control measures. Leaf-vegetables and rice were primarily polluted by Cd and Pb. The main four sources of heavy metals in soils were traffic emission, metal smelting, agricultural activities and natural sources, mining extraction, and electroplating industries. Heavy metals with the highest ecological risk and health risk are Cd and As, respectively. The non-carcinogenic and carcinogenic risks of children were 7.0 and 1.7 times higher than those of adults, respectively. Therefore, children are more likely to be influenced by heavy metals compared to adults. The results obtained by the risk assessments may contribute to the identification of specific sources of heavy metals (e.g., traffic emissions, metal smelting, mining excavation, and electroplating industries). Additionally, the environmental impacts and biotoxicity associated with various heavy metals (e.g., Cd and As) can also be reflected. These outcomes may serve as a scientific basis for the pollution monitoring and remediation in the mining-affected areas.
近年来,由于潜在风险的存在,中国土壤重金属污染已成为一个主要关注点。为了评估江西省一个典型重金属污染场地的环境污染和人体健康风险,本研究对羊眉江流域土壤中重金属的分布、污染水平和来源进行了全面评估。本研究采用正定矩阵因子分解和蒙特卡罗模拟评价重金属的生态和人体健康风险。研究结果表明,土壤中 20-40cm 深处重金属污染最严重,局部重金属污染是由采矿和污水灌溉造成的。高风险区占总面积的 91.11%。然而,由于采样效应、降雨和控制措施的影响,污染水平随时间降低。叶菜类和水稻主要受到 Cd 和 Pb 的污染。土壤中重金属的主要四个来源是交通排放、金属冶炼、农业活动和自然源、采矿和电镀工业。土壤中生态风险和健康风险最高的重金属分别是 Cd 和 As。儿童的非致癌和致癌风险分别是成人的 7.0 倍和 1.7 倍,因此,儿童比成人更容易受到重金属的影响。风险评估结果可能有助于识别重金属的具体来源(如交通排放、金属冶炼、采矿和电镀工业)。此外,还可以反映各种重金属(如 Cd 和 As)的环境影响和生物毒性。这些结果可以为矿区污染监测和修复提供科学依据。