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中国煤矿和金属矿区土壤潜在有毒元素污染的主要影响因素识别及概率健康风险评估:系统评价。

Major influencing factors identification and probabilistic health risk assessment of soil potentially toxic elements pollution in coal and metal mines across China: A systematic review.

机构信息

College of Water Sciences, Beijing Normal University, Beijing 100875, China; State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.

Technical Centre for Soil, Agriculture and Rural Ecology and Environment, Ministry of Ecology and Environment, Beijing 100012, China.

出版信息

Ecotoxicol Environ Saf. 2024 Apr 1;274:116231. doi: 10.1016/j.ecoenv.2024.116231. Epub 2024 Mar 19.

Abstract

Deposition of potentially toxic elements (PTEs) in soils due to different types of mining activities has been an increasingly important concern worldwide. Quantitative differences of soil PTEs contamination and related health risk among typical mines remain unclear. Herein, data from 110 coal mines and 168 metal mines across China were analyzed based on 265 published literatures to evaluate pollution characteristics, spatial distribution, and probabilistic health risks of soil PTEs. The results showed that PTE levels in soil from both mine types significantly exceeded background values. The geoaccumulation index (I) revealed metal-mine soil pollution levels exceeded those of coal mines, with average I values for Cd, Hg, As, Pb, Cu, and Zn being 3.02-15.60 times higher. Spearman correlation and redundancy analysis identified natural and anthropogenic factors affecting soil PTE contamination in both mine types. Mining activities posed a significant carcinogenic risk, with metal-mine soils showing a total carcinogenic risk an order of magnitude higher than in coal-mine soils. This study provides policymakers a quantitative foundation for developing differentiated strategies for sustainable remediation and risk-based management of PTEs in typical mining soils.

摘要

由于不同类型的采矿活动,土壤中潜在有毒元素(PTEs)的沉积已成为全球日益关注的问题。典型矿山土壤 PTE 污染的定量差异以及相关健康风险仍不清楚。在此,基于 265 篇已发表文献,对中国 110 个煤矿和 168 个金属矿的数据进行了分析,以评估土壤 PTE 的污染特征、空间分布和概率健康风险。结果表明,两种类型矿山的土壤中 PTE 水平均显著高于背景值。地积累指数(I)表明金属矿山土壤污染水平超过了煤矿,Cd、Hg、As、Pb、Cu 和 Zn 的平均 I 值分别高出 3.02-15.60 倍。Spearman 相关和冗余分析确定了影响两种类型矿山土壤 PTE 污染的自然和人为因素。采矿活动造成了显著的致癌风险,金属矿山土壤的总致癌风险比煤矿土壤高一个数量级。本研究为决策者制定差异化策略提供了定量依据,以实现典型矿山土壤中 PTE 的可持续修复和基于风险的管理。

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