Pang Chunlin, Li Fei, Hu Xiaorao, Meng Keyu, Pan Hong, Xiang Yong
School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu, 611731, China.
School of Electronic and Information Engineering, Changchun University, Changchun, 130022, China.
Discov Nano. 2024 Mar 25;19(1):55. doi: 10.1186/s11671-024-04001-z.
Degradable wearable electronics are attracting increasing attention to weaken or eliminate the negative effect of waste e-wastes and promote the development of medical implants without secondary post-treatment. Although various degradable materials have been explored for wearable electronics, the development of degradable wearable electronics with integrated characteristics of highly sensing performances and low-cost manufacture remains challenging. Herein, we developed a facile, low-cost, and environmentally friendly approach to fabricate a biocompatible and degradable silk fibroin based wearable electronics (SFWE) for on-body monitoring. A combination of rose petal templating and hollow carbon nanospheres endows as-fabricated SFWE with good sensitivity (5.63 kPa), a fast response time (147 ms), and stable durability (15,000 cycles). The degradable phenomenon has been observed in the solution of 1 M NaOH, confirming that silk fibroin based wearable electronics possess degradable property. Furthermore, the as-fabricated SFWE have been demonstrated that have abilities to monitor knuckle bending, muscle movement, and facial expression. This work offers an ecologically-benign and cost-effective approach to fabricate high-performance wearable electronics.
可降解可穿戴电子设备正受到越来越多的关注,以减轻或消除废弃电子垃圾的负面影响,并促进无需二次后处理的医用植入物的发展。尽管已经为可穿戴电子设备探索了各种可降解材料,但开发具有高传感性能和低成本制造集成特性的可降解可穿戴电子设备仍然具有挑战性。在此,我们开发了一种简便、低成本且环保的方法来制造用于人体监测的生物相容性和可降解的丝素蛋白基可穿戴电子设备(SFWE)。玫瑰花瓣模板法与中空碳纳米球相结合,使制备的SFWE具有良好的灵敏度(5.63 kPa)、快速响应时间(147 ms)和稳定的耐久性(15000次循环)。在1 M NaOH溶液中观察到了降解现象,证实了丝素蛋白基可穿戴电子设备具有可降解性能。此外,已证明制备的SFWE具有监测指关节弯曲、肌肉运动和面部表情的能力。这项工作提供了一种生态友好且经济高效的方法来制造高性能可穿戴电子设备。