Univ Lyon, Université Claude Bernard Lyon 1, CNRS, ENTPE, UMR 5023 LEHNA, F-69518, Vaulx-en-Velin, France; INSA Lyon, DEEP, EA 7429, 69621, Villeurbanne, France.
Univ Lyon, Université Claude Bernard Lyon 1, CNRS, ENTPE, UMR 5023 LEHNA, F-69518, Vaulx-en-Velin, France.
Environ Pollut. 2024 May 1;348:123882. doi: 10.1016/j.envpol.2024.123882. Epub 2024 Mar 26.
The assessment of microplastic (MP) pollution in urban areas is essential considering its abundance in freshwater, particularly due to urban wet weather discharge. The precise sources of MPs must be identified to better understand its characteristics. This study examines the relationship between MP pollution in detention basin sediments and land use in the investigated catchments. The study of stormwater management infrastructure, mainly in detention basins, has enabled the quantification of MP abundance in sediments conveyed by stormwater in urban areas. Sediment sampling was conducted in ten detention basins and one combined sewer overflow (CSO) structure in the Lyon metropolitan area, France. These basins correspond to stormwater outlets of representative urban catchment areas. MP extraction involves densimetric separation and organic matter degradation. MPs were then characterized using micro-Fourier infrared spectroscopy and siMPle software. This protocol identified MPs between 50 and 500 μm in the study sites. This study highlights the high abundance in the collected sediment samples, ranging from 2,525 to 1,218,82 MP kg by dry weight sediment. The MPs found have a median size around 115 μm, making them very small MPs that are mainly composed of polypropylene followed by polyethylene and polystyrene or polyethylene terephthalate. The abundance of MPs in sediments is associated with the land use type. Catchments in predominantly industrial and commercial zones were more significantly polluted with MPs compared with those in predominantly agricultural or heterogeneous zones. Finally, statistical analyses revealed links between sedimentary and urban parameters and MPs concentrations. Several recommendations are given for future research, notably concerning the analyzing of stormwater sediments to understand the sources of MP pollution.
考虑到城市地区淡水中微塑料(MP)污染的丰富程度,特别是由于城市湿天气排放,评估其污染至关重要。必须确定 MPs 的精确来源,以更好地了解其特征。本研究考察了截留盆地沉积物中 MP 污染与研究流域土地利用之间的关系。对雨水管理基础设施的研究,主要是截留盆地,使我们能够量化城市地区雨水输送沉积物中 MP 的丰度。在法国里昂大都市区的十个截留盆地和一个合流制溢流(CSO)结构中进行了沉积物采样。这些盆地对应于具有代表性的城市集水区的雨水出口。MP 提取涉及密度分离和有机物降解。然后使用微傅里叶红外光谱和 siMPle 软件对 MPs 进行了特征描述。该方案在研究地点确定了 50 至 500μm 之间的 MPs。本研究强调了在收集的沉积物样本中含量高,从 2525 到 121882 MPs kg 干重沉积物不等。发现的 MPs 的中值尺寸约为 115μm,使其成为主要由聚丙烯组成的非常小的 MPs,其次是聚乙烯和聚苯乙烯或聚对苯二甲酸乙二醇酯。沉积物中 MPs 的丰度与土地利用类型有关。与主要是农业或异质区的流域相比,主要是工业和商业区的流域受 MPs 污染更为严重。最后,统计分析揭示了沉积物和城市参数与 MPs 浓度之间的联系。为未来的研究提出了一些建议,特别是关于分析雨水沉积物以了解 MP 污染的来源。