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将活性物质从晶体固体塑造为活性湍流。

Shaping active matter from crystalline solids to active turbulence.

作者信息

Yang Qianhong, Jiang Maoqiang, Picano Francesco, Zhu Lailai

机构信息

Department of Mechanical Engineering, National University of Singapore, Singapore, Singapore.

School of Naval Architecture, Ocean and Energy Power Engineering, Wuhan University of Technology, Wuhan, Hubei, PR China.

出版信息

Nat Commun. 2024 Apr 3;15(1):2874. doi: 10.1038/s41467-024-46520-4.

Abstract

Active matter drives its constituent agents to move autonomously by harnessing free energy, leading to diverse emergent states with relevance to both biological processes and inanimate functionalities. Achieving maximum reconfigurability of active materials with minimal control remains a desirable yet challenging goal. Here, we employ large-scale, agent-resolved simulations to demonstrate that modulating the activity of a wet phoretic medium alone can govern its solid-liquid-gas phase transitions and, subsequently, laminar-turbulent transitions in fluid phases, thereby shaping its emergent pattern. These two progressively emerging transitions, hitherto unreported, bring us closer to perceiving the parallels between active matter and traditional matter. Our work reproduces and reconciles seemingly conflicting experimental observations on chemically active systems, presenting a unified landscape of phoretic collective dynamics. These findings enhance the understanding of long-range, many-body interactions among phoretic agents, offer new insights into their non-equilibrium collective behaviors, and provide potential guidelines for designing reconfigurable materials.

摘要

活性物质通过利用自由能驱动其组成成分自主移动,从而产生与生物过程和无生命功能相关的各种涌现状态。以最小的控制实现活性材料的最大可重构性仍然是一个理想但具有挑战性的目标。在此,我们采用大规模、基于个体的模拟来证明,仅调节湿电泳介质的活性就可以控制其固-液-气相变,进而控制流体相中的层流-湍流转变,从而塑造其涌现模式。这两个逐渐出现的转变,迄今尚未见报道,使我们更接近于认识活性物质与传统物质之间的相似之处。我们的工作重现并调和了关于化学活性系统看似相互矛盾的实验观察结果,呈现出电泳集体动力学的统一图景。这些发现加深了对电泳粒子间长程多体相互作用的理解,为其非平衡集体行为提供了新的见解,并为设计可重构材料提供了潜在的指导原则。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ca95/11258367/8c3f458be448/41467_2024_46520_Fig1_HTML.jpg

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