Wu Wen-Ya, Zhang Mingsheng, Wang Cun, Tao Longgang, Bu Jie, Zhu Qiang
Institute of Materials Research and Engineering (IMRE), Agency for Science, Technology and Research (A*STAR), 2 Fusionopolis Way, Innovis #08-03, Singapore, 138634, Republic of Singapore.
Institute of Sustainability for Chemicals, Energy and Environment (ISCE2), Agency for Science, Technology and Research (A*STAR), 1 Pesek Road, Jurong Island, Singapore, 627833, Republic ofSingapore.
Chem Asian J. 2024 Jun 17;19(12):e202400180. doi: 10.1002/asia.202400180. Epub 2024 May 17.
This review explores the potential of using different types of ash, namely fly ash, biomass ash, and coal ash etc., as mediums for CO capture and sequestration. The diverse origins of these ash types - municipal waste, organic biomass, and coal combustion - impart unique physicochemical properties that influence their suitability and efficiency in CO absorption. This review first discusses the environmental and economic implications of using ash wastes, emphasizing the reduction in landfill usage and the transformation of waste into value-added products. Then the chemical/physical treatments of ash wastes and their inherent capabilities in binding or reacting with CO are introduced, along with current methodologies utilize these ashes for CO sequestration, including mineral carbonation and direct air capture techniques. The application of using ash wastes for CO capture are highlighted, followed by the discussion regarding challenges associated with ash-based CO absorption approach. Finally, the article projects into the future, proposing innovative approaches and technological advancements needed to enhance the efficacy of ash in combating the increasing CO levels. By providing a comprehensive analysis of current strategies and envisioning future prospects, this review aims to contribute to the field of sustainable CO absorption and environmental management.
本综述探讨了使用不同类型的灰分(即粉煤灰、生物质灰和煤灰等)作为二氧化碳捕获和封存介质的潜力。这些灰分类型的来源多样——城市垃圾、有机生物质和煤炭燃烧——赋予了它们独特的物理化学性质,这些性质影响着它们在二氧化碳吸收方面的适用性和效率。本综述首先讨论了使用灰分废弃物的环境和经济意义,强调减少填埋场使用以及将废弃物转化为增值产品。然后介绍了灰分废弃物的化学/物理处理方法及其与二氧化碳结合或反应的固有能力,以及目前利用这些灰分进行二氧化碳封存的方法,包括矿物碳酸化和直接空气捕获技术。重点介绍了使用灰分废弃物进行二氧化碳捕获的应用,随后讨论了基于灰分的二氧化碳吸收方法所面临的挑战。最后,本文展望未来,提出了提高灰分在应对不断上升的二氧化碳水平方面的功效所需的创新方法和技术进步。通过对当前策略进行全面分析并展望未来前景,本综述旨在为可持续二氧化碳吸收和环境管理领域做出贡献。