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利用源自生物质原料的活性炭强化二氧化碳捕集的综合综述。

A comprehensive review of enhanced CO capture using activated carbon derived from biomass feedstock.

作者信息

Kundu Shreyase, Khandaker Tasmina, Anik Md Al-Amin Mia, Hasan Md Kamrul, Dhar Palash Kumar, Dutta Sagar Kumar, Latif M Abdul, Hossain Muhammad Sarwar

机构信息

Chemistry Discipline, Khulna University Khulna-9208 Bangladesh

Department of Chemistry, Bangladesh Army University of Engineering & Technology (BAUET) Qadirabad Cantonment Natore-6431 Bangladesh.

出版信息

RSC Adv. 2024 Sep 18;14(40):29693-29736. doi: 10.1039/d4ra04537h. eCollection 2024 Sep 12.

DOI:10.1039/d4ra04537h
PMID:39297049
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11409178/
Abstract

The increasing level of atmospheric CO requires the urgent development of effective capture technologies. This comprehensive review thoroughly examines various methods for the synthesis of carbon materials, modification techniques for converting biomass feedstock into carbon materials and pivotal factors impacting their properties. The novel aspect of this review is its in-depth comparison of how these modifications specifically affect the pore structure and surface area together with the exploration of the mechanism underlying the enhancement of CO adsorption performance. Additionally, this review addresses research gaps and provides recommendations for future studies concerning the advantages and drawbacks of CO adsorbents and their prospects for commercialization and economic feasibility. This article revealed that among the various strategies, template carbonization offers a viable option for providing control of the material pore diameter and structure without additional modification treatments. Optimizing the pore structure of activated carbons, particularly those activated with agents such as KOH and ZnCl, together with synthesizing hybrid activated carbons using multiple activating agents, is crucial for enhancing their CO capture performance. Cost-benefit analysis suggests that biomass-derived activated carbons can significantly meet the escalating demand for CO capture materials, offering economic advantages and supporting sustainable waste management.

摘要

大气中二氧化碳（CO）水平的不断上升，迫切需要开发有效的捕集技术。本综述全面研究了碳材料合成的各种方法、将生物质原料转化为碳材料的改性技术以及影响其性能的关键因素。本综述的新颖之处在于深入比较了这些改性如何具体影响孔隙结构和表面积，并探讨了提高CO吸附性能的潜在机制。此外，本综述还指出了研究空白，并针对CO吸附剂的优缺点及其商业化前景和经济可行性提供了未来研究的建议。本文表明，在各种策略中，模板碳化提供了一种可行的选择，无需额外的改性处理即可控制材料的孔径和结构。优化活性炭的孔隙结构，特别是那些用KOH和ZnCl等试剂活化的活性炭，以及使用多种活化剂合成混合活性炭，对于提高其CO捕集性能至关重要。成本效益分析表明，生物质衍生的活性炭能够显著满足对CO捕集材料不断增长的需求，具有经济优势并支持可持续的废物管理。

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