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智能超级电容器中基于金属有机框架/氧化石墨烯的复合材料：关于先进储能器件的电化学评估和材料开发的全面综述

MOF/graphene oxide based composites in smart supercapacitors: a comprehensive review on the electrochemical evaluation and material development for advanced energy storage devices.

作者信息

Gautam Sanjeev, Rialach Shruti, Paul Surinder, Goyal Navdeep

机构信息

Advanced Functional Materials Lab, Dr S.S. Bhatnagar University Institute of Chemical Engineering & Technology, Panjab University Chandigarh-160014 India

Department of Physics and Astronomical Science, Central University of Himachal Pradesh Dharamshala 176215 India.

出版信息

RSC Adv. 2024 Apr 30;14(20):14311-14339. doi: 10.1039/d4ra01027b. eCollection 2024 Apr 25.

DOI:10.1039/d4ra01027b
PMID:38690108
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11060142/
Abstract

The surge in interest surrounding energy storage solutions, driven by the demand for electric vehicles and the global energy crisis, has spotlighted the effectiveness of carbon-based supercapacitors in meeting high-power requirements. Concurrently, metal-organic frameworks (MOFs) have gained attention as a template for their integration with graphene oxide (GO) in composite materials which have emerged as a promising avenue for developing high-power supercapacitors, elevating smart supercapacitor efficiency, cyclic stability, and durability, providing crucial insights for overcoming contemporary energy storage obstacles. The identified combination leverages the strengths of both materials, showcasing significant potential for advancing energy storage technologies in a sustainable and efficient manner. In this research, an in-depth review has been presented, in which properties, rationale and integration of MOF/GO composites have been critically examined. Various fabrication techniques have been thoroughly analyzed, emphasizing the specific attributes of MOFs, such as high surface area and modifiable porosity, in tandem with the conductive and stabilizing features of graphene oxide. Electrochemical characterizations and physicochemical mechanisms underlying MOF/GO composites have been examined, emphasizing their synergistic interaction, leading to superior electrical conductivity, mechanical robustness, and energy storage capacity. The article concludes by identifying future research directions, emphasizing sustainable production, material optimization, and integration strategies to address the persistent challenges in the field of energy storage. In essence, this research article aims to offer a concise and insightful resource for researchers engaged in overcoming the pressing energy storage issues of our time through the exploration of MOF/GO composites in smart supercapacitors.

摘要

受电动汽车需求和全球能源危机的推动，围绕储能解决方案的兴趣激增，凸显了碳基超级电容器在满足高功率需求方面的有效性。与此同时，金属有机框架（MOF）作为一种模板受到关注，可将其与氧化石墨烯（GO）整合到复合材料中，这已成为开发高功率超级电容器、提高智能超级电容器效率、循环稳定性和耐久性的一条有前景的途径，为克服当代储能障碍提供了关键见解。所确定的组合利用了两种材料的优势，展示了以可持续和高效方式推进储能技术的巨大潜力。在本研究中，进行了深入综述，对MOF/GO复合材料的性能、原理和整合进行了批判性研究。全面分析了各种制备技术，强调了MOF的特定属性，如高表面积和可调节的孔隙率，以及氧化石墨烯的导电和稳定特性。研究了MOF/GO复合材料的电化学表征和物理化学机制，强调了它们的协同相互作用，从而带来卓越的导电性、机械强度和储能能力。文章最后确定了未来的研究方向，强调可持续生产、材料优化和整合策略，以应对储能领域持续存在的挑战。本质上，这篇研究文章旨在为研究人员提供一份简洁而有见地的资源，通过探索智能超级电容器中的MOF/GO复合材料来克服我们这个时代紧迫的储能问题。

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