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光催化生产过氧化氢的最新进展。

Recent developments in photocatalytic production of hydrogen peroxide.

作者信息

Fang Xiao, Huang Xi, Hu Qiyu, Li Bonan, Hu Chunlian, Ma Baochun, Ding Yong

机构信息

State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Advanced Catalysis of Gansu Province, College of Chemistry and Chemical Engineering, Lanzhou University, 222 Tianshui South Road, Lanzhou 730000, China.

State Key Laboratory of Low Carbon Catalysis and Carbon Dioxide Utilization, State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, 18 Tianshui Middle Road, Lanzhou 730000, China.

出版信息

Chem Commun (Camb). 2024 May 16;60(41):5354-5368. doi: 10.1039/d4cc01577k.

Abstract

Hydrogen peroxide (HO), an environmentally friendly strong oxidant and energy carrier, has attracted widespread attention in photocatalysis. Artificial photosynthesis of HO using water and oxygen as raw materials, solar energy as an energy source, and semiconductor materials as catalysts is considered a promising technology. In the past few decades, encouraging progress has been made in the photocatalytic production of HO. Therefore, we summarize the research achievements in this field in recent years. This review first briefly introduces the reaction pathway, detection techniques and evaluation metrics. Then, the recent advances in photocatalysts are highlighted. Furthermore, the existing challenges and possible solutions in this field are presented. At last, we look forward to the future development direction of this field. This review provides valuable insights and guidance for efficient photocatalytic HO production.

摘要

过氧化氢(HO)作为一种环境友好型强氧化剂和能量载体,在光催化领域受到了广泛关注。以水和氧气为原料、太阳能为能源、半导体材料为催化剂进行HO的人工光合作用被认为是一项很有前景的技术。在过去几十年里,HO的光催化生产取得了令人鼓舞的进展。因此,我们总结了近年来该领域的研究成果。本综述首先简要介绍了反应途径、检测技术和评估指标。然后,重点介绍了光催化剂的最新进展。此外,还阐述了该领域目前存在的挑战及可能的解决方案。最后,我们展望了该领域未来的发展方向。本综述为高效光催化生产HO提供了有价值的见解和指导。

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