• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利：CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法，用中文像聊天一样搜索，搜遍4000万医学文献。AI智能推荐，让科研检索更轻松。

立即免费搜索

文件翻译

保留排版，准确专业，支持PDF/Word/PPT等文件格式，支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述，25分钟生成高质量综述，智能提取关键信息，辅助科研写作。

立即免费体验

用于有机染料降解的多孔珊瑚状氧化锌纳米片的光催化效率增强

Enhanced photocatalytic efficiency of porous ZnO coral-like nanoplates for organic dye degradation.

作者信息

Hanh Nguyen Hong, Thi Minh Nguyet Quan, Van Chinh Tran, Duong La Duc, Xuan Tien Tran, Van Duy Lai, Hoa Nguyen Duc

机构信息

Institute of Engineering Physics, Academy of Military Science and Technology 17 Hoang Sam Street, Cau Giay District Hanoi City Vietnam

School of Engineering Physics, Hanoi University of Science and Technology (HUST) No. 1 Dai Co Viet Street Hanoi City Vietnam.

出版信息

RSC Adv. 2024 May 3;14(21):14672-14679. doi: 10.1039/d4ra01345j. eCollection 2024 May 2.

DOI:10.1039/d4ra01345j
PMID:38708121
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11067434/
Abstract

ZnO nanomaterials have been extensively used as photocatalysts for the removal of pollutants in aqueous environments. This study explores the enhanced photocatalytic performance of porous ZnO coral-like nanoplates synthesized a one-pot wet-chemical method and subsequent annealing treatment. Characterization through scanning electron microscopy (SEM), high-resolution transmission electron microscopy (HRTEM), powder X-ray diffraction (XRD), energy-dispersive X-ray spectroscopy (EDX), Raman spectroscopy, photoluminescence (PL) spectroscopy, and Brunauer-Emmett-Teller (BET) measurements confirmed the nanoplates' porous structure, single-crystal structure, 100 nm thickness, and 80 nm pore size. These unique structural characteristics of the ZnO coral-like nanoplates enabled effective photodegradation of the organic dye rhodamine B (RhB) under visible light irradiation. Under simulated sunlight, the ZnO photocatalyst exhibited exceptional performance, achieving a 97.3% removal rate of RhB after 210 minutes of irradiation. The prepared ZnO photocatalyst also showed remarkable photostability and regeneration capability for RhB photodegradation with a decreased efficiency of less than 15% after eight testing cycles. The potential mechanism of the ZnO photocatalyst toward RhB degradation was also studied and is discussed in detail.

摘要

氧化锌纳米材料已被广泛用作光催化剂，用于去除水环境中的污染物。本研究探索了通过一锅湿化学法合成及后续退火处理制备的多孔氧化锌珊瑚状纳米片增强的光催化性能。通过扫描电子显微镜（SEM）、高分辨率透射电子显微镜（HRTEM）、粉末X射线衍射（XRD）、能量色散X射线光谱（EDX）、拉曼光谱、光致发光（PL）光谱和布鲁诺尔-埃米特-泰勒（BET）测量进行表征，证实了纳米片的多孔结构、单晶结构、100nm的厚度和80nm的孔径。氧化锌珊瑚状纳米片的这些独特结构特征使得其在可见光照射下能够有效地光降解有机染料罗丹明B（RhB）。在模拟太阳光下，氧化锌光催化剂表现出优异的性能，在照射210分钟后，罗丹明B的去除率达到97.3%。所制备的氧化锌光催化剂还表现出显著的光稳定性和罗丹明B光降解的再生能力，在八个测试循环后效率降低不到15%。还研究了氧化锌光催化剂对罗丹明B降解的潜在机制，并进行了详细讨论。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/9cb755d849b1/d4ra01345j-f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/5c0a8598f422/d4ra01345j-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/ec9c9521a695/d4ra01345j-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/f67a85d66b4a/d4ra01345j-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/07cc09f13066/d4ra01345j-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/87e4c98fab0b/d4ra01345j-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/5c76bef87218/d4ra01345j-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/b5c904d90df0/d4ra01345j-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/9cb755d849b1/d4ra01345j-f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/5c0a8598f422/d4ra01345j-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/ec9c9521a695/d4ra01345j-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/f67a85d66b4a/d4ra01345j-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/07cc09f13066/d4ra01345j-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/87e4c98fab0b/d4ra01345j-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/5c76bef87218/d4ra01345j-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/b5c904d90df0/d4ra01345j-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9b37/11067434/9cb755d849b1/d4ra01345j-f8.jpg

相似文献

1
Enhanced photocatalytic efficiency of porous ZnO coral-like nanoplates for organic dye degradation.用于有机染料降解的多孔珊瑚状氧化锌纳米片的光催化效率增强
RSC Adv. 2024 May 3;14(21):14672-14679. doi: 10.1039/d4ra01345j. eCollection 2024 May 2.
2
Coupling ZnO with CuO for efficient organic pollutant removal.将 ZnO 与 CuO 耦合用于高效去除有机污染物。
Environ Sci Pollut Res Int. 2023 Jun;30(28):71984-72008. doi: 10.1007/s11356-022-24139-6. Epub 2022 Nov 22.
3
In-Situ Hydrothermal Fabrication of ZnO-Loaded GAC Nanocomposite for Efficient Rhodamine B Dye Removal via Synergistic Photocatalytic and Adsorptive Performance.原位水热法制备负载氧化锌的颗粒活性炭纳米复合材料，通过协同光催化和吸附性能高效去除罗丹明B染料
Nanomaterials (Basel). 2024 Jul 22;14(14):1234. doi: 10.3390/nano14141234.
4
Enhanced visible light photodegradation activity of RhB/MB from aqueous solution using nanosized novel Fe-Cd co-modified ZnO.使用纳米级新型铁-镉共修饰氧化锌增强水溶液中罗丹明B/亚甲基蓝的可见光光降解活性。
Sci Rep. 2018 Jul 16;8(1):10691. doi: 10.1038/s41598-018-29025-1.
5
A magnetically separable plate-like cadmium titanate-copper ferrite nanocomposite with enhanced visible-light photocatalytic degradation performance for organic contaminants.一种具有增强的可见光光催化降解有机污染物性能的磁性可分离板状钛酸镉-铜铁氧体纳米复合材料。
RSC Adv. 2019 May 17;9(27):15615-15628. doi: 10.1039/c9ra01968e. eCollection 2019 May 14.
6
Photocatalytic, sonocatalytic and sonophotocatalytic degradation of Rhodamine B using ZnO/CNTs composites photocatalysts.采用 ZnO/CNTs 复合材料光催化剂对 Rhodamine B 进行光催化、声催化和超声光催化降解。
Ultrason Sonochem. 2014 Mar;21(2):761-73. doi: 10.1016/j.ultsonch.2013.08.014. Epub 2013 Aug 30.
7
Facile synthesis of porous single crystalline ZnO nanoplates and their application in photocatalytic reduction of Cr(VI) in the presence of phenol.多孔单晶 ZnO 纳米片的简便合成及其在苯酚存在下光催化还原 Cr(VI)中的应用。
J Hazard Mater. 2014 Jul 15;276:400-7. doi: 10.1016/j.jhazmat.2014.05.059. Epub 2014 May 29.
8
Fabrication of SrTiO anchored rGO/g-CN photocatalyst for the removal of mixed dye from wastewater: dual photocatalytic mechanism.用于去除废水中混合染料的 SrTiO 锚定 rGO/g-CN 光催化剂的制备：双光催化机制
Sci Rep. 2024 Jul 15;14(1):16259. doi: 10.1038/s41598-024-66844-x.
9
Green synthesis of CuO/FeO/ZnO ternary composite photocatalyst using grape extract for enhanced photodegradation of environmental organic pollutant.利用葡萄提取物绿色合成CuO/FeO/ZnO三元复合光催化剂用于增强环境有机污染物的光降解
Chemosphere. 2024 Mar;351:141212. doi: 10.1016/j.chemosphere.2024.141212. Epub 2024 Jan 19.
10
Enhanced photocatalytic degradation of malachite green using manganese oxide doped graphene oxide/zinc oxide (GO-ZnO/MnO) ternary composite under sunlight irradiation.在阳光照射下，使用氧化锰掺杂的氧化石墨烯/氧化锌（GO-ZnO/MnO）三元复合材料增强孔雀石绿的光催化降解。
J Environ Manage. 2022 Sep 15;318:115449. doi: 10.1016/j.jenvman.2022.115449. Epub 2022 Jun 17.

本文引用的文献

1
Recent advancements in the fabrication and photocatalytic applications of graphitic carbon nitride-tungsten oxide nanocomposites.石墨相氮化碳-氧化钨纳米复合材料的制备及其光催化应用的最新进展
Nanoscale Adv. 2023 Aug 21;5(19):5214-5255. doi: 10.1039/d3na00159h. eCollection 2023 Sep 26.
2
A Review on Photocatalysis Used For Wastewater Treatment: Dye Degradation.用于废水处理的光催化：染料降解综述
Water Air Soil Pollut. 2023;234(6):349. doi: 10.1007/s11270-023-06359-9. Epub 2023 May 26.
3
Facile preparation of porphyrin@g-CN/Ag nanocomposite for improved photocatalytic degradation of organic dyes in aqueous solution.
卟啉@g-CN/Ag 纳米复合材料的简便制备及其在水溶液中对有机染料的光催化降解性能的改善。
Environ Res. 2023 Aug 15;231(Pt 1):115984. doi: 10.1016/j.envres.2023.115984. Epub 2023 May 6.
4
Impact on the Photocatalytic Dye Degradation of Morphology and Annealing-Induced Defects in Zinc Oxide Nanostructures.形貌及退火诱导缺陷对氧化锌纳米结构光催化染料降解的影响
ACS Omega. 2023 Apr 17;8(17):14952-14964. doi: 10.1021/acsomega.2c07412. eCollection 2023 May 2.
5
Engineering S-scheme CuO/ZnO heterojunctions sonochemically for eradicating RhB dye from wastewater under solar radiation.通过超声化学方法制备工程化S型CuO/ZnO异质结以在太阳辐射下从废水中去除罗丹明B染料。
RSC Adv. 2023 Apr 28;13(19):13269-13281. doi: 10.1039/d3ra00924f. eCollection 2023 Apr 24.
6
Photocatalytic Performance of Undoped and Al-Doped ZnO Nanoparticles in the Degradation of Rhodamine B under UV-Visible Light:The Role of Defects and Morphology.无掺杂和 Al 掺杂 ZnO 纳米粒子在紫外-可见光下降解罗丹明 B 的光催化性能：缺陷和形态的作用。
Int J Mol Sci. 2022 Dec 7;23(24):15459. doi: 10.3390/ijms232415459.
7
Highly efficient catalytic/sonocatalytic reduction of 4-nitrophenol and antibacterial activity through a bifunctional Ag/ZnO nanohybrid material prepared a sodium alginate method.通过海藻酸钠法制备的双功能Ag/ZnO纳米杂化材料实现对4-硝基苯酚的高效催化/声催化还原及抗菌活性
Nanoscale Adv. 2019 Jul 2;1(8):3151-3163. doi: 10.1039/c9na00075e. eCollection 2019 Aug 6.
8
Fabrication of Ag/ZnO@N-Carbon Core@Shell Photocatalyst for Efficient Photocatalytic Degradation of Rhodamine B.用于高效光催化降解罗丹明B的Ag/ZnO@N-碳核壳光催化剂的制备
Front Chem. 2022 Jun 30;10:950007. doi: 10.3389/fchem.2022.950007. eCollection 2022.
9
Impact of atomic layer deposited TiO on the photocatalytic efficiency of TiO/w-VA-CNT nanocomposite materials.原子层沉积TiO对TiO/w-VA-CNT纳米复合材料光催化效率的影响。
RSC Adv. 2022 Jun 1;12(26):16419-16430. doi: 10.1039/d1ra09410f.
10
Self-Assembly of Porphyrin Nanofibers on ZnO Nanoparticles for the Enhanced Photocatalytic Performance for Organic Dye Degradation.卟啉纳米纤维在氧化锌纳米颗粒上的自组装用于增强光催化降解有机染料的性能
ACS Omega. 2021 Sep 2;6(36):23203-23210. doi: 10.1021/acsomega.1c02808. eCollection 2021 Sep 14.