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基于镉/铅量子点敏化太阳能电池电解质开发的近期进展综述：性能与稳定性

Review of recent progress in the development of electrolytes for Cd/Pb-based quantum dot-sensitized solar cells: performance and stability.

作者信息

Kasaye Bayisa Batu, Shura Megersa Wodajo, Dibaba Solomon Tiruneh

机构信息

Department of Applied Physics, School of Natural and Applied Sciences, Adama Science and Technology University Adama Oromia Ethiopia

出版信息

RSC Adv. 2024 May 20;14(23):16255-16268. doi: 10.1039/d4ra01030b. eCollection 2024 May 15.

DOI:10.1039/d4ra01030b
PMID:38769954
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11103669/
Abstract

Quantum dot-sensitized solar cells (QDSSCs) represent an exciting advancement in third-generation photovoltaic solar cells owing to their ability to generate multiple electron-hole pairs per photon, high stability under light and moisture exposure, and flexibility in size and composition tuning. Although these cells have achieved power conversion efficiencies exceeding 15%, there remains a challenge in enhancing both their efficiency and stability for practical large-scale applications. Therefore, in this review, we aimed to investigate recent progress in improving the long-term stability, analyzing the impact of advanced quantum dot properties on charge-transport optimization, and assessing the role of interface engineering in reducing recombination losses to maximize QDSSC performance and stability. Additionally, this review delves into key elements such as the electrolyte composition, ionic conductivity, and compatibility with counter electrodes and photoanodes to understand their influence on power conversion efficiencies and stability. Finally, potential directions for advancing QDSC development in future are discussed to provide insights into the obstacles and opportunities for achieving high-efficiency QDSSCs.

摘要

量子点敏化太阳能电池（QDSSCs）是第三代光伏太阳能电池领域一项令人振奋的进展，这得益于其能够每吸收一个光子就产生多个电子 - 空穴对、在光照和潮湿环境下具有高稳定性以及在尺寸和成分调整方面具有灵活性。尽管这些电池已经实现了超过15%的功率转换效率，但在提高其效率和稳定性以实现实际大规模应用方面仍存在挑战。因此，在本综述中，我们旨在研究在提高长期稳定性方面的最新进展，分析先进量子点特性对电荷传输优化的影响，并评估界面工程在减少复合损失以最大化QDSSC性能和稳定性方面的作用。此外，本综述深入探讨了诸如电解质组成、离子电导率以及与对电极和光阳极的兼容性等关键要素，以了解它们对功率转换效率和稳定性的影响。最后，讨论了未来推进量子点敏化太阳能电池发展的潜在方向，以便深入了解实现高效QDSSCs所面临的障碍和机遇。

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