Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University, 4-101 minami, Koyama-cho, Tottori 680-8552, Japan.
Center for Research on Green Sustainable Chemistry, Tottori University, 4-101 minami, Koyama-cho, Tottori 680-8552, Japan.
ACS Appl Bio Mater. 2024 Jun 17;7(6):3629-3635. doi: 10.1021/acsabm.4c00494. Epub 2024 May 31.
We prepared composite electrodes using TiO coated with chlorophylls and as photoelectric conversion material and MnO as energy storage material and investigated their photoelectrochemical capacitor properties. The coating with the combination of chlorophylls and improved the photoelectric conversion function of TiO, compared with the coating with each alone. Na adsorption on MnO was enhanced with increasing the chlorophyll coating amount. The reason is that more chlorophylls and absorb visible light in different wavelengths to promote an easier photoexcited electron transfer to MnO, just as they improve the efficiency of photosynthesis reactions in nature.
我们制备了 TiO 复合电极,以叶绿素 和 作为光电转换材料,以 MnO 作为储能材料,并研究了它们的光电化学电容器性能。与单独涂覆相比,叶绿素 和 的组合涂覆提高了 TiO 的光电转换功能。随着叶绿素涂覆量的增加,MnO 上的 Na 吸附增强。原因是更多的叶绿素 和 吸收不同波长的可见光,促进光激发电子更容易转移到 MnO,就像它们提高了自然界光合作用反应的效率一样。