Tabataba-Vakili Farsane, Nguyen Huy P G, Rupp Anna, Mosina Kseniia, Papavasileiou Anastasios, Watanabe Kenji, Taniguchi Takashi, Maletinsky Patrick, Glazov Mikhail M, Sofer Zdenek, Baimuratov Anvar S, Högele Alexander
Fakultät für Physik, Munich Quantum Center, and Center for NanoScience (CeNS), Ludwig-Maximilians-Universität München, Geschwister-Scholl-Platz 1, 80539, München, Germany.
Munich Center for Quantum Science and Technology (MCQST), 80799, München, Germany.
Nat Commun. 2024 Jun 3;15(1):4735. doi: 10.1038/s41467-024-49048-9.
Magnetism in two-dimensional materials reveals phenomena distinct from bulk magnetic crystals, with sensitivity to charge doping and electric fields in monolayer and bilayer van der Waals magnet CrI. Within the class of layered magnets, semiconducting CrSBr stands out by featuring stability under ambient conditions, correlating excitons with magnetic order and thus providing strong magnon-exciton coupling, and exhibiting peculiar magneto-optics of exciton-polaritons. Here, we demonstrate that both exciton and magnetic transitions in bilayer and trilayer CrSBr are sensitive to voltage-controlled field-effect charging, exhibiting bound exciton-charge complexes and doping-induced metamagnetic transitions. Moreover, we demonstrate how these unique properties enable optical probes of local magnetic order, visualizing magnetic domains of competing phases across metamagnetic transitions induced by magnetic field or electrostatic doping. Our work identifies few-layer CrSBr as a rich platform for exploring collaborative effects of charge, optical excitations, and magnetism.
二维材料中的磁性揭示了与块状磁性晶体不同的现象,在单层和双层范德华磁体CrI₃中对电荷掺杂和电场敏感。在层状磁体类别中,半导体CrSBr脱颖而出,它在环境条件下具有稳定性,将激子与磁序相关联,从而提供强的磁振子-激子耦合,并表现出激子极化激元的奇特磁光特性。在这里,我们证明双层和三层CrSBr中的激子和磁跃迁对电压控制的场效应充电敏感,表现出束缚激子-电荷复合体和掺杂诱导的变磁跃迁。此外,我们展示了这些独特性质如何实现对局部磁序的光学探测,可视化由磁场或静电掺杂诱导的变磁跃迁中竞争相的磁畴。我们的工作确定了少层CrSBr是探索电荷、光学激发和磁性协同效应的丰富平台。