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拓扑螺旋链衍生的边缘态观察。

Observation of edge states derived from topological helix chains.

机构信息

Department of Physics, Tohoku University, Sendai, Japan.

Precursory Research for Embryonic Science and Technology (PRESTO), Japan Science and Technology Agency (JST), Tokyo, Japan.

出版信息

Nature. 2024 Jul;631(8019):54-59. doi: 10.1038/s41586-024-07484-z. Epub 2024 Jun 5.

DOI:10.1038/s41586-024-07484-z
PMID:38839966
Abstract

Introducing the concept of topology has revolutionized materials classification, leading to the discovery of topological insulators and Dirac-Weyl semimetals. One of the most fundamental theories underpinning topological materials is the Su-Schrieffer-Heeger (SSH) model, which was developed in 1979-decades before the recognition of topological insulators-to describe conducting polymers. Distinct from the vast majority of known topological insulators with two and three dimensions, the SSH model predicts a one-dimensional analogue of topological insulators, which hosts topological bound states at the endpoints of a chain. To establish this unique and pivotal state, it is crucial to identify the low-energy excitations stemming from bound states, but this has remained unknown in solids because of the absence of suitable platforms. Here we report unusual electronic states that support the emergent bound states in elemental tellurium, the single helix of which was recently proposed to realize an extended version of the SSH chain. Using spin- and angle-resolved photoemission spectroscopy with a micro-focused beam, we have shown spin-polarized in-gap states confined to the edges of the (0001) surface. Our density functional theory calculations indicate that these states are attributed to the interacting bound states originating from the one-dimensional array of SSH tellurium chains. Helices in solids offer a promising experimental platform for investigating exotic properties associated with the SSH chain and exploring topological phases through dimensionality control.

摘要

引入拓扑概念彻底改变了材料分类,导致拓扑绝缘体和狄拉克-外尔半金属的发现。支撑拓扑材料的最基本理论之一是 Su-Schrieffer-Heeger(SSH)模型,该模型于 1979 年开发,早于拓扑绝缘体的发现,用于描述导电聚合物。与绝大多数具有二维和三维的已知拓扑绝缘体不同,SSH 模型预测了拓扑绝缘体的一维类似物,在链的端点处存在拓扑束缚态。为了建立这种独特而关键的状态,必须识别源于束缚态的低能激发,但由于缺乏合适的平台,这在固体中仍然未知。在这里,我们报告了在元素碲中支持新兴束缚态的不寻常电子态,其单一螺旋结构最近被提议实现 SSH 链的扩展版本。我们使用具有微聚焦光束的自旋和角度分辨光发射光谱,已经证明了局限于(0001)表面边缘的自旋极化带内态。我们的密度泛函理论计算表明,这些状态归因于源自一维 SSH 碲链阵列的相互作用束缚态。固体中的螺旋结构为研究与 SSH 链相关的奇异性质以及通过维度控制探索拓扑相提供了一个很有前途的实验平台。

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本文引用的文献

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Development of Ar gas cluster ion beam system for surface preparation in angle-resolved photoemission spectroscopy.用于角分辨光电子能谱表面准备的 Ar 气体团束离子源系统的开发。
Rev Sci Instrum. 2023 Feb 1;94(2):023904. doi: 10.1063/5.0100610.
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Topological phase change transistors based on tellurium Weyl semiconductor.基于碲化外尔半导体的拓扑相变晶体管。
Sci Adv. 2022 Jun 10;8(23):eabn3837. doi: 10.1126/sciadv.abn3837.
3
Development of a versatile micro-focused angle-resolved photoemission spectroscopy system with Kirkpatrick-Baez mirror optics.
采用柯克帕特里克-贝兹镜光学系统的多功能微聚焦角分辨光电子能谱系统的研制。
Rev Sci Instrum. 2022 Mar 1;93(3):033906. doi: 10.1063/5.0074393.
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Phase transition and topological transistors based on monolayer NaBi nanoribbons.基于单层NaBi纳米带的相变与拓扑晶体管
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Radial Spin Texture of the Weyl Fermions in Chiral Tellurium.手性碲中狄拉克费米子的径向自旋纹理
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1D topological phases in transition-metal monochalcogenide nanowires.过渡金属硫族化合物纳米线中的一维拓扑相
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Radial Spin Texture in Elemental Tellurium with Chiral Crystal Structure.具有手性晶体结构的元素碲中的径向自旋纹理。
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