Tang Haotian, Stan Liliana, Czaplewski David A, Yang Xiaodong, Gao Jie
Opt Express. 2024 May 20;32(11):20136-20145. doi: 10.1364/OE.525756.
Integrating phase-change materials in metasurfaces has emerged as a powerful strategy to realize optical devices with tunable electromagnetic responses. Here, phase-change chiral metasurfaces based on GST-225 material with the designed trapezoid-shaped resonators are demonstrated to achieve tunable circular dichroism (CD) responses in the infrared regime. The asymmetric trapezoid-shaped resonators are designed to support two chiral plasmonic resonances with opposite CD responses for realizing switchable CD between negative and positive values using the GST phase change from amorphous to crystalline. The electromagnetic field distributions of the chiral plasmonic resonant modes are analyzed to understand the chiroptical responses of the metasurface. Furthermore, the variations in the absorption spectrum and CD value for the metasurface as a function of the baking time during the GST phase transition are analyzed to reveal the underlying thermal tuning process of the metasurface. The demonstrated phase-change metasurfaces with tunable CD responses hold significant promise in enabling many applications in the infrared regime such as chiral sensing, encrypted communication, and thermal imaging.
将相变材料集成到超表面已成为实现具有可调谐电磁响应的光学器件的有力策略。在此,展示了基于GST-225材料且带有设计的梯形谐振器的相变手性超表面,以在红外波段实现可调谐圆二色性(CD)响应。设计不对称梯形谐振器以支持具有相反CD响应的两种手性等离子体共振,从而利用GST从非晶态到晶态的相变实现正负值之间可切换的CD。分析手性等离子体共振模式的电磁场分布,以了解超表面的手性光学响应。此外,分析了超表面在GST相变期间吸收光谱和CD值随烘烤时间的变化,以揭示超表面潜在的热调谐过程。所展示的具有可调谐CD响应的相变超表面在实现红外波段的许多应用(如手性传感、加密通信和热成像)方面具有巨大潜力。