Browne Christopher A, Datta Sujit S
Department of Chemical and Biological Engineering, Princeton University, Princeton, NJ 08544.
Proc Natl Acad Sci U S A. 2024 Jul 16;121(29):e2320962121. doi: 10.1073/pnas.2320962121. Epub 2024 Jul 9.
Turbulent flows have been used for millennia to mix solutes; a familiar example is stirring cream into coffee. However, many energy, environmental, and industrial processes rely on the mixing of solutes in porous media where confinement suppresses inertial turbulence. As a result, mixing is drastically hindered, requiring fluid to permeate long distances for appreciable mixing and introducing additional steps to drive mixing that can be expensive and environmentally harmful. Here, we demonstrate that this limitation can be overcome just by adding dilute amounts of flexible polymers to the fluid. Flow-driven stretching of the polymers generates an elastic instability, driving turbulent-like chaotic flow fluctuations, despite the pore-scale confinement that prohibits typical inertial turbulence. Using in situ imaging, we show that these fluctuations stretch and fold the fluid within the pores along thin layers ("lamellae") characterized by sharp solute concentration gradients, driving mixing by diffusion in the pores. This process results in a [Formula: see text] reduction in the required mixing length, a [Formula: see text] increase in solute transverse dispersivity, and can be harnessed to increase the rate at which chemical compounds react by [Formula: see text]-enhancements that we rationalize using turbulence-inspired modeling of the underlying transport processes. Our work thereby establishes a simple, robust, versatile, and predictive way to mix solutes in porous media, with potential applications ranging from large-scale chemical production to environmental remediation.
湍流用于混合溶质已有数千年历史;一个常见的例子是将奶油搅拌到咖啡中。然而,许多能源、环境和工业过程依赖于溶质在多孔介质中的混合,而在多孔介质中,受限环境会抑制惯性湍流。因此,混合受到极大阻碍,需要流体渗透很长距离才能实现可观的混合,并引入额外的驱动混合步骤,这些步骤可能成本高昂且对环境有害。在此,我们证明,只需向流体中添加少量柔性聚合物就能克服这一限制。聚合物在流动驱动下的拉伸会产生弹性不稳定性,从而驱动类似湍流的混沌流动波动,尽管孔隙尺度的限制会阻止典型的惯性湍流。通过原位成像,我们表明这些波动会沿着以尖锐溶质浓度梯度为特征的薄层(“薄片”)拉伸和折叠孔隙内的流体,通过孔隙内的扩散驱动混合。这一过程使所需的混合长度减少了[公式:见原文],溶质横向扩散率提高了[公式:见原文],并且可用于通过[公式:见原文]增强化学反应速率,我们通过对基础传输过程进行受湍流启发的建模来解释这种增强。我们的工作由此建立了一种简单、稳健、通用且可预测的方法来在多孔介质中混合溶质,其潜在应用范围从大规模化学生产到环境修复。