Dong Yuyang, Arai Yosuke, Kuroda Kenta, Ochi Masayuki, Tanaka Natsumi, Wan Yuxuan, Watson Matthew D, Kim Timur K, Cacho Cephise, Hashimoto Makoto, Lu Donghui, Aoki Yuji, Matsuda Tatsuma D, Kondo Takeshi
Institute for Solid State Physics, <a href="https://ror.org/057zh3y96">The University of Tokyo</a>, Kashiwa, Chiba 277-8581, Japan.
Graduate School of Advanced Science and Engineering, <a href="https://ror.org/03t78wx29">Hiroshima University</a>, Higashi-hiroshima, Hiroshima 739-8526, Japan.
Phys Rev Lett. 2024 Jul 5;133(1):016401. doi: 10.1103/PhysRevLett.133.016401.
The magnetic skyrmions generated in a centrosymmetric crystal were recently first discovered in Gd_{2}PdSi_{3}. In light of this, we observe the electronic structure by angle-resolved photoemission spectroscopy and unveil its direct relationship with the magnetism in this compound. The Fermi surface and band dispersions are demonstrated to have a good agreement with the density functional theory calculations carried out with careful consideration of the crystal superstructure. Most importantly, we find that the three-dimensional Fermi surface has extended nesting which matches well the q vector of the magnetic order detected by recent scattering measurements. The consistency we find among angle-resolved photoemission spectroscopy, density functional theory, and the scattering measurements suggests the Ruderman-Kittel-Kasuya-Yosida interaction involving itinerant electrons to be the formation mechanism of skyrmions in Gd_{2}PdSi_{3}.
最近在中心对称晶体中产生的磁斯格明子首次在Gd₂PdSi₃中被发现。鉴于此,我们通过角分辨光电子能谱观察其电子结构,并揭示其与该化合物磁性的直接关系。费米面和能带色散被证明与在仔细考虑晶体超结构的情况下进行的密度泛函理论计算有很好的一致性。最重要的是,我们发现三维费米面具有扩展嵌套,这与最近散射测量检测到的磁有序q矢量很好地匹配。我们在角分辨光电子能谱、密度泛函理论和散射测量之间发现的一致性表明,涉及巡游电子的Ruderman-Kittel-Kasuya-Yosida相互作用是Gd₂PdSi₃中斯格明子的形成机制。