钌纳米颗粒与Ni-N(O)-C位点之间的相互作用诱导的电子再分布促进了碱性水电解。
Electronic redistribution induced by interaction between ruthenium nanoparticles and Ni-N(O)-C sites boosts alkaline water electrolysis.
作者信息
Wang Jiacheng, He Wangtao, Zong Yuyang, Tang Yanfeng, Wang Jin, Ma Ruguang
机构信息
Zhejiang Key Laboratory for Island Green Energy and New Materials, Institute of Electrochemistry, School of Materials Science and Engineering, Taizhou University, Taizhou 318000, Zhejiang, China.
State Key Laboratory of High-Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China.
出版信息
Chem Commun (Camb). 2024 Aug 27;60(70):9444-9447. doi: 10.1039/d4cc02851a.
Ultrafine ruthenium nanoparticles are encapsulated by single-atom Ni-bonded graphitic carbon nitride (g-CN) layers anchored on carbon nanotubes (Ru/Ni-CNCT). The enhanced electronic interaction between Ru nanoparticles and Ni-N(O)-C sites anchored in g-CN layers promotes water adsorption/dissociation and hydrogen evolution.
超细钌纳米颗粒被锚定在碳纳米管上的单原子镍键合石墨相氮化碳（g-CN）层包裹（Ru/Ni-CNCT）。钌纳米颗粒与锚定在g-CN层中的Ni-N(O)-C位点之间增强的电子相互作用促进了水的吸附/解离和析氢反应。
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