Institute of Marine Science and Technology, Shandong University, Qingdao, 266237, China; Shandong Engineering Research Center for Environmental Protection and Remediation on Groundwater, Jinan, 250014, China.
Institute of Marine Science and Technology, Shandong University, Qingdao, 266237, China.
Chemosphere. 2024 Sep;364:143185. doi: 10.1016/j.chemosphere.2024.143185. Epub 2024 Aug 24.
The Landfill plays an important role in urban development and waste disposal. However, landfill leachate may also bring more serious pollution and health risks to the surrounding groundwater environment. Compared with other areas, the area around the landfill needs more precise management. To solve this problem, based on the "pressure-state-response" framework, a method for the identification and evaluation of groundwater pollution around the landfill was constructed. The LPI method was used to assess the contamination potential of the leachate. The comprehensive quality of groundwater was evaluated by the entropy-AHP water quality assessment method, sodium adsorption ratio and sodium percentage. The probabilistic health risks of groundwater were assessed based on a Monte Carlo algorithm. The sources of pollutants were identified by comprehensively using the PCA-APCS-MLR model and the PMF model. Finally, the self-organizing map algorithm and the Kmeans algorithm were integrated to enhance the precision of groundwater management and control measures. The results showed that the leachate of the landfill was in the mature stage, and the concentration of inorganic substances was relatively high. Leachate had the potential to contaminate surrounding groundwater. The groundwater quality of 68.14% of the study area was in the poor or lower level. The groundwater near the landfill was unsuitable not only for drinking but also for irrigation purposes. Cl was the main non-carcinogenic risk factor. Reducing pollutant concentration and controlling exposure time are effective strategies for mitigating health risks caused by high-concentration pollutants (Cl, NO) and low-concentration pollutants (F), respectively. The groundwater around the landfill was jointly affected by six pollution sources. The PMF model has better analytical ability in mixed pollution areas. The groundwater in the study area was divided into five clusters, of which cluster Ⅰ was significantly affected by leachate, and cluster Ⅴ had the lowest pollution and health risk.
垃圾填埋场在城市发展和废物处理中起着重要作用。然而,垃圾渗滤液也可能给周围地下水环境带来更严重的污染和健康风险。与其他地区相比,垃圾填埋场周围地区需要更精确的管理。为了解决这个问题,基于“压力-状态-响应”框架,构建了一种用于识别和评估垃圾填埋场周围地下水污染的方法。利用 LPI 方法评估渗滤液的污染潜力。利用熵-AHP 水质评价法、钠吸附比和钠百分比综合评价地下水综合质量。基于蒙特卡罗算法评估地下水的概率健康风险。综合利用 PCA-APCS-MLR 模型和 PMF 模型识别污染物来源。最后,整合自组织映射算法和 Kmeans 算法,提高地下水管理和控制措施的精度。结果表明,垃圾填埋场的渗滤液处于成熟阶段,无机物质浓度相对较高。渗滤液有污染周围地下水的潜力。研究区 68.14%的地下水水质处于较差或更低水平。垃圾填埋场附近的地下水不仅不适合饮用,也不适合灌溉。Cl 是主要的非致癌风险因素。降低污染物浓度和控制暴露时间是减轻高浓度污染物(Cl、NO)和低浓度污染物(F)引起的健康风险的有效策略。垃圾填埋场周围的地下水受到六个污染源的共同影响。PMF 模型在混合污染区域具有更好的分析能力。研究区地下水分为五个聚类,其中聚类Ⅰ受渗滤液影响显著,聚类Ⅴ污染和健康风险最低。