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通过光图案化实现对三维孤立波的控制。

Command of three-dimensional solitary waves via photopatterning.

作者信息

Li Chao-Yi, Tang Xing-Zhou, Yu Xiao, Atzin Noe, Song Zhen-Peng, Chen Chu-Qiao, Abbott Nicholas L, Li Bing-Xiang, de Pablo Juan J, Lu Yan-Qing

机构信息

National Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China.

College of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology), Nanjing University of Posts and Telecommunications, Nanjing 210023, China.

出版信息

Proc Natl Acad Sci U S A. 2024 Sep 3;121(36):e2405168121. doi: 10.1073/pnas.2405168121. Epub 2024 Aug 28.

DOI:10.1073/pnas.2405168121
PMID:39196620
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11388288/
Abstract

Multidimensional solitons are prevalent in numerous research fields. In orientationally ordered soft matter system, three-dimensional director solitons exemplify the localized distortion of molecular orientation. However, their precise manipulation remains challenging due to unpredictable and uncontrolled generation. Here, we utilize preimposed programmable photopatterning in nematics to control the kinetics of director solitons. This enables both unidirectional and bidirectional generation at specific locations and times, confinement within micron-scaled patterns of diverse shapes, and directed propagation along predefined trajectories. A focused dynamical model provides insight into the origins of these solitons and aligns closely with experimental observations, underscoring the pivotal role of anchoring conditions in soliton manipulation. Our findings pave the way for diverse fundamental research avenues and promising applications, including microcargo transportation and optical information processing.

摘要

多维孤子在众多研究领域中普遍存在。在取向有序的软物质系统中,三维指向矢孤子体现了分子取向的局部畸变。然而,由于其产生具有不可预测性和不可控性,对它们进行精确操控仍然具有挑战性。在此,我们利用向列相液晶中预先施加的可编程光图案化来控制指向矢孤子的动力学。这使得在特定位置和时间实现单向和双向产生、限制在各种形状的微米级图案内以及沿预定轨迹的定向传播成为可能。一个聚焦的动力学模型揭示了这些孤子的起源,并与实验观测结果紧密吻合,强调了锚定条件在孤子操控中的关键作用。我们的研究结果为包括微载体运输和光学信息处理在内的各种基础研究途径和有前景的应用铺平了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/aa460783369c/pnas.2405168121fig06.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/dd6a801a2c5e/pnas.2405168121fig01.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/258f0825d2d4/pnas.2405168121fig02.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/fcb8b2c6b053/pnas.2405168121fig03.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/4f4def8c59e1/pnas.2405168121fig04.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/8522dd6d2403/pnas.2405168121fig05.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/aa460783369c/pnas.2405168121fig06.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/dd6a801a2c5e/pnas.2405168121fig01.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/258f0825d2d4/pnas.2405168121fig02.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/fcb8b2c6b053/pnas.2405168121fig03.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/4f4def8c59e1/pnas.2405168121fig04.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/8522dd6d2403/pnas.2405168121fig05.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9fcf/11388288/aa460783369c/pnas.2405168121fig06.jpg

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本文引用的文献

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Field-controlled dynamics of skyrmions and monopoles.斯格明子和磁单极子的场控动力学
Sci Adv. 2024 Jan 26;10(4):eadj9373. doi: 10.1126/sciadv.adj9373.
3
Minimal Model of Solitons in Nematic Liquid Crystals.向列型液晶中孤子的最小模型
Phys Rev Lett. 2023 Nov 3;131(18):188101. doi: 10.1103/PhysRevLett.131.188101.
4
Jetting and Droplet Formation Driven by Interfacial Electrohydrodynamic Effects Mediated by Solitons in Liquid Crystals.由液晶中孤子介导的界面电流体动力学效应驱动的喷射和液滴形成
Phys Rev Lett. 2023 Sep 1;131(9):098101. doi: 10.1103/PhysRevLett.131.098101.
5
Programming Solitons in Liquid Crystals Using Surface Chemistry.利用表面化学在液晶中编程孤子
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Design of nematic liquid crystals to control microscale dynamics.用于控制微观尺度动力学的向列型液晶设计。
Liq Cryst Rev. 2020;8(2):59-129. doi: 10.1080/21680396.2021.1919576. Epub 2021 May 26.
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