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通过与共轭的2,4,6-三氨基嘧啶-g-CN构建异质结提高ZnO纳米线的光催化性能

Boosting Photocatalytic Performance of ZnO Nanowires via Building Heterojunction with Conjugated 2,4,6-Triaminopyrimidine-g-CN.

作者信息

Lou Jiahui, Wang Lihong, Huang Yaqiong, Xing Jun, Yang Xiaojie

机构信息

Hubei Key Laboratory of Radiation Chemistry and Functional Materials, School of Nuclear Technology and Chemistry & Biology, Hubei University of Science and Technology, Xianning 437100, China.

School of Biomedical Engineering and Imaging, Hubei University of Science and Technology, Xianning 437100, China.

出版信息

Molecules. 2024 Aug 6;29(16):3716. doi: 10.3390/molecules29163716.

Abstract

Photocatalysis is one of the most effective ways to solve environmental problems by solving pollutants. This article designed and prepared a conjugated system of 2,4,6-triaminopyrimidine-g-CN (TAP-CN) to modify ZnO NWs. We systematically studied the photocatalytic performance of ZnO NWs modified with different ratios of TAP-CN. The results showed that 9 wt% TAP-CN-30/ZnO NWs had the best degradation effect on Rhodamine B dye. The degradation rate was 99.36% in 80 min. The excellent degradation performance was attributed to the TAP-CN conjugated system promoting photo-generated charge transfer. This work provided guidance for designing efficient composite catalysts for application in other renewable energy fields.

摘要

光催化是通过解决污染物来解决环境问题的最有效方法之一。本文设计并制备了2,4,6-三氨基嘧啶-g-CN(TAP-CN)共轭体系以修饰ZnO纳米线。我们系统地研究了不同比例TAP-CN修饰的ZnO纳米线的光催化性能。结果表明,9 wt% TAP-CN-30/ZnO纳米线对罗丹明B染料具有最佳降解效果。80分钟内降解率为99.36%。优异的降解性能归因于TAP-CN共轭体系促进光生电荷转移。这项工作为设计用于其他可再生能源领域的高效复合催化剂提供了指导。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9304/11356989/f24054443633/molecules-29-03716-g001.jpg

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