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离子液体催化的一氧化碳转化制备高价值化学品

Ionic Liquid-Catalyzed CO Conversion for Valuable Chemicals.

作者信息

Wang Peng, Wang Rui

机构信息

School of Environmental Science and Engineering, Shandong University, No. 72 Seaside Road, Qingdao 266237, China.

出版信息

Molecules. 2024 Aug 11;29(16):3805. doi: 10.3390/molecules29163805.

DOI:10.3390/molecules29163805
PMID:39202884
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11357070/
Abstract

CO is not only the main gas that causes the greenhouse effect but also a resource with abundant reserves, low price, and low toxicity. It is expected to become an important "carbon source" to replace oil and natural gas in the future. The efficient and clean resource utilization of CO has shown important scientific and economic value. Making full use of abundant CO resources is in line with the development direction of green chemistry and has attracted the attention of scientists. Environmentally friendly ionic liquids show unique advantages in the capture and conversion of CO due to their non-volatilization, designable structure, and good solubility, and show broad application prospects. The purpose of this paper is to discuss the research on the use of an ionic liquid as a catalyst to promote the synthesis of various value-added chemicals in CO, hoping to make full use of CO resources while avoiding the defects of the traditional synthesis route, such as the use of highly toxic raw materials, complicated operation, or harsh reaction conditions. The purpose of this paper is to provide reference for the application and development of ionic liquids in CO capture and conversion.

摘要

一氧化碳不仅是造成温室效应的主要气体,也是一种储量丰富、价格低廉、毒性较低的资源。预计未来它将成为替代石油和天然气的重要“碳源”。一氧化碳的高效清洁资源利用已显示出重要的科学和经济价值。充分利用丰富的一氧化碳资源符合绿色化学的发展方向,已引起科学家们的关注。环境友好型离子液体由于其不挥发、结构可设计和良好的溶解性,在一氧化碳的捕获和转化方面显示出独特优势,并展现出广阔的应用前景。本文旨在探讨使用离子液体作为催化剂促进一氧化碳中各种增值化学品合成的研究,希望在充分利用一氧化碳资源的同时,避免传统合成路线存在的使用剧毒原料、操作复杂或反应条件苛刻等缺陷。本文旨在为离子液体在一氧化碳捕获和转化中的应用与发展提供参考。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/6352914d9156/molecules-29-03805-g010.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/2bfd72975e84/molecules-29-03805-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/12adf5391285/molecules-29-03805-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/423b701c8b05/molecules-29-03805-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/0db503ddb0ea/molecules-29-03805-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/93c818a1bf69/molecules-29-03805-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/4a84b8bdc2c5/molecules-29-03805-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/f6d009fb4f58/molecules-29-03805-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/f776533f95b5/molecules-29-03805-g008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/c7e34a77b48c/molecules-29-03805-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/6352914d9156/molecules-29-03805-g010.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/2bfd72975e84/molecules-29-03805-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/12adf5391285/molecules-29-03805-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/423b701c8b05/molecules-29-03805-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/0db503ddb0ea/molecules-29-03805-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/93c818a1bf69/molecules-29-03805-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/4a84b8bdc2c5/molecules-29-03805-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/f6d009fb4f58/molecules-29-03805-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/f776533f95b5/molecules-29-03805-g008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/c7e34a77b48c/molecules-29-03805-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c427/11357070/6352914d9156/molecules-29-03805-g010.jpg

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Designing Copper-Based Catalysts for Efficient Carbon Dioxide Electroreduction.设计用于高效二氧化碳电还原的铜基催化剂。
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