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油页岩原位催化转化催化剂的最新进展

Recent Progress on In Situ Catalytic Conversion Catalysts for Oil Shale.

作者信息

Wu Aibin, Wu Junwen, Chen Liu, Su Jianzheng, Yu Weichu

机构信息

State Key Laboratory of Shale Oil and Gas Enrichment Mechanisms and Effective Development, Beijing 102206, P.R. China.

State Center for Research and Development of Oil Shale Exploitation, Beijing 102206, P.R. China.

出版信息

ACS Omega. 2024 Aug 22;9(35):36904-36916. doi: 10.1021/acsomega.4c04724. eCollection 2024 Sep 3.

DOI:10.1021/acsomega.4c04724
PMID:39246466
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11375725/
Abstract

With the gradual depletion of oil resources, it is urgent to vigorously develop unconventional and renewable energy sources. As an unconventional resource with abundant resources, the rational and efficient development of oil shale is of great significance to alleviating the national energy crisis. The main methods of oil shale development are surface dry distillation and in situ transformation. In situ catalytic conversion technology, as an emerging mining method, has the potential to improve efficiency, reduce costs, and environmental impact and is an important direction for future oil shale development. As a key component in the in situ conversion process, catalysts play a crucial role in the rate, selectivity, and product quality of the reaction. However, the research on oil shale pyrolysis catalysts is still in the laboratory stage and is difficult to translate into practical applications. Therefore, this paper reviews recent progress of catalyst research in the in situ catalytic conversion of oil shale, including the types, design principles, and reaction mechanisms of catalysts, and looks forward to the future development direction. It provides a certain reference for the discovery of new catalysts that can improve yield and reduce environmental pollution in the process of oil shale extraction and also provides a valuable technical reference for the green development and utilization of unconventional and strategic alternative energy sources in the world and the transformation and sustainable development of the global energy structure.

摘要

随着石油资源的逐渐枯竭，大力发展非常规和可再生能源迫在眉睫。油页岩作为一种资源丰富的非常规资源，其合理高效开发对缓解国家能源危机具有重要意义。油页岩开发的主要方法是地表干馏和原位转化。原位催化转化技术作为一种新兴的开采方法，具有提高效率、降低成本和环境影响的潜力，是未来油页岩开发的重要方向。作为原位转化过程中的关键组成部分，催化剂在反应速率、选择性和产品质量方面起着至关重要的作用。然而，油页岩热解催化剂的研究仍处于实验室阶段，难以转化为实际应用。因此，本文综述了油页岩原位催化转化中催化剂研究的最新进展，包括催化剂的类型、设计原理和反应机理，并展望了未来的发展方向。它为发现能够提高油页岩开采过程中产量并减少环境污染的新型催化剂提供了一定参考，也为世界非常规和战略替代能源的绿色开发利用以及全球能源结构的转型和可持续发展提供了有价值的技术参考。

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Ir-CoO Active Centers Supported on Porous Al O Nanosheets as Efficient and Durable Photo-Thermal Catalysts for CO Conversion.负载在多孔 Al2O3 纳米片上的 Ir-CoO 活性中心作为高效且耐用的 CO 转化光热催化剂。
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