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关中地区典型煤矿区土壤中潜在有毒元素(PTEs)的来源识别及生态与概率健康风险的系统评估

Systematic assessment of source identification and ecological and probabilistic health risks of potentially toxic elements (PTEs) in soils of a typical coal mining area in Guanzhong region.

作者信息

Chen Daokun, Li Xinbin, Wang Zhanbin, Kang Chengxin, He Tao, Liu Hanyuan, Jiang Zhiyang, Xi Junsheng, Zhang Yao

机构信息

Xi'an Center of Mineral Resources Survey, China Geological Survery, Xi'an, 710100, China.

School of Earth and Environment, Anhui University of Science & Technology, Huainan, 232001, China.

出版信息

Heliyon. 2024 Aug 16;10(17):e36301. doi: 10.1016/j.heliyon.2024.e36301. eCollection 2024 Sep 15.

DOI:10.1016/j.heliyon.2024.e36301
PMID:39263165
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11387233/
Abstract

Mining activities may cause the accumulation of potentially toxic elements (PTEs) in surrounding soils, posing ecological threats and health dangers to the local population. Therefore, a comprehensive assessment using multiple indicators was used to quantify the level of risk in the region. The results showed that the mean values of the nine potentially toxic elements in the study area were lower than the background values only for Cr, and the lowest coefficient of variation was 17.1 % for As, and the spatial distribution characteristics of the elements indicate that they are enriched by different factors. The elements Hg and Cd, which have substantial cumulative features, are the key contributors to ecological risk in the study region, which is overall at moderate risk. APCS-MLR model parses out 4 possible sources: mixed industrial, mining and transportation sources (53.98 %), natural sources (24.56 %), atmospheric deposition sources (12.60 %), and agricultural production sources (8.76 %). The probabilistic health risks show that children are more susceptible to health risks than adults; among children, the safety criteria (HI < 1 and CR < 10) were surpassed by 29.29 % of THI and 8.58 % of TCR. According to source-orientated health hazards, the element Ni significantly increases the risk of cancer. Mixed sources from industry, mining, and transportation are important sources of health risks. The results of this research provide some scientific references for the management and decrease of regional ecological and health risks.

摘要

采矿活动可能导致周围土壤中潜在有毒元素(PTEs)的积累,对当地居民构成生态威胁和健康危害。因此,采用综合多指标评估方法来量化该地区的风险水平。结果表明,研究区域内9种潜在有毒元素的平均值仅铬低于背景值,变异系数最低的是砷,为17.1%,元素的空间分布特征表明它们受不同因素富集。具有显著累积特征的汞和镉元素是研究区域生态风险的主要贡献者,该区域总体处于中等风险水平。APCS-MLR模型解析出4种可能的来源:混合工业、采矿和交通源(53.98%)、自然源(24.56%)、大气沉降源(12.60%)和农业生产源(8.76%)。概率健康风险表明,儿童比成人更容易受到健康风险影响;在儿童中,29.29%的THI和8.58%的TCR超过了安全标准(HI < 1且CR < 10)。根据源导向的健康危害,镍元素显著增加癌症风险。工业、采矿和交通的混合源是健康风险的重要来源。本研究结果为区域生态和健康风险的管理与降低提供了一些科学参考。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/88617fb3b04d/gr8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/aee101d95c3b/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/6747029415c6/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/18b3aaebee80/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/6eddad01a715/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/dc4fe7e30766/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/83a2fbb7993e/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/d2e89e093593/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/88617fb3b04d/gr8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/aee101d95c3b/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/6747029415c6/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/18b3aaebee80/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/6eddad01a715/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/dc4fe7e30766/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/83a2fbb7993e/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/d2e89e093593/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6ae4/11387233/88617fb3b04d/gr8.jpg

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