Mentes Dóra, Jordán Anikó, Farkas László, Muránszky Gábor, Fiser Béla, Viskolcz Béla, Póliska Csaba
Institute of Energy and Quality, University of Miskolc, 3515, Miskolc, Miskolc-Egyetemváros, Hungary.
Higher Education and Industrial Cooperation Centre, University of Miskolc, 3515, Miskolc-Egyetemváros, Hungary.
Sci Rep. 2024 Sep 12;14(1):21314. doi: 10.1038/s41598-024-72173-w.
In Europe mainly at winter season the PM levels exceed air quality limits, which correlated with the operation of solid-fired boilers. More and more people are returning to using these devices due to energy shortage caused by the pandemic and regional conflicts. In addition, the phenomena of co-burning fuels and municipal waste in residential boilers in primarily fuel poverty households increases further the amount of pollutants in the atmosphere. This study aims to correlate the quantity and quality of air pollutants with the type of fuel (wood and wastes) burned. Combustion experiments were conducted using oak fuel mixed with three waste groups: (1) plastics (PP, HDPE, PET); (2) textiles (polyester-PES, cotton-COT); and (3) papers (cardboard-CARD, glossy coated paper-GCP, 84C/PAP). The addition of waste to wood fuel altered the morphology of emitted particles. While waste burning doesn't always increase particle quantity, it significantly raises PAH concentrations. A strong relationship exists between waste type, particle morphology, and PAH quality, where with lower molecular weight PAHs linked to tar agglomerates and higher ones to soot agglomerates with inorganic crystals.
在欧洲,主要在冬季,细颗粒物(PM)水平超过空气质量限值,这与固体燃料锅炉的运行相关。由于疫情和地区冲突导致能源短缺,越来越多的人重新开始使用这些设备。此外,在主要处于燃料贫困的家庭中,住宅锅炉中燃料与城市垃圾共燃的现象进一步增加了大气中的污染物数量。本研究旨在将空气污染物的数量和质量与燃烧的燃料类型(木材和废物)相关联。使用与三类废物混合的橡木燃料进行了燃烧实验:(1)塑料(聚丙烯、高密度聚乙烯、聚对苯二甲酸乙二酯);(2)纺织品(聚酯、棉);以及(3)纸张(硬纸板、光面涂层纸、84克/纸)。向木材燃料中添加废物改变了排放颗粒的形态。虽然废物燃烧并不总是增加颗粒数量,但它显著提高了多环芳烃(PAH)浓度。废物类型、颗粒形态和多环芳烃质量之间存在很强的关系,其中低分子量多环芳烃与焦油团聚物相关,而高分子量多环芳烃与含有无机晶体的烟灰团聚物相关。