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具有“星爆涡轮”设计的太阳能驱动蒸发器,具有定向盐结晶、抗菌和催化多功能性,用于高效水净化。

Solar-Driven Evaporator With "Starburst Turbine" Design Featuring Directional Salt Crystallization, Antibacterial, and Catalytic Multifunctionality for Efficient Water Purification.

作者信息

Yu Jiahui, Li Lele, Liu Yuxuan, Wen Jie, Liu Shu, Li Jiye, Ning Junyi, Shao Changxiang, Wu Tao, Liu Bing

机构信息

Department of Stomatology, Shandong Provincial Hospital Affiliated to Shandong First Medical University, Jinan, 250021, China.

Medical Science and Technology Innovation Center, School of Stomatology, Shandong First Medical University & Shandong Academy of Medical Sciences, Jinan, 250117, China.

出版信息

Adv Sci (Weinh). 2024 Nov;11(43):e2406696. doi: 10.1002/advs.202406696. Epub 2024 Sep 25.

DOI:10.1002/advs.202406696
PMID:39320342
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11578366/
Abstract

Facing the global challenge of water scarcity, solar-driven desalination is considered a sustainable technology for obtaining freshwater from seawater. However, issues such as uncontrolled salt crystallization and bacterial contamination limit its efficiency and practicality. This study proposes an innovative solar-driven evaporator designed to address these challenges using optimized shape design and advanced photothermal materials. Based on finite element analyses, cylindrical evaporators with a "Starburst Turbine" shape are designed and fabricated, achieving directional salt crystallization and a record-breaking water collection rate of 3.56 kg m h and an evaporation rate of 4.57 kg m h under one sun illumination. During continuous 60-h illumination tests, the evaporator maintained a stable evaporation rate, attributed to its excellent directional salt crystallization capability. Additionally, the evaporator demonstrates superior photodynamic antibacterial performance and photocatalytic degradation of organic pollutants. Under one sun illumination for 1 h, it achieves 100% sterilization of S. aureus and E. coli, and a 95.4% degradation of methylene blue (MB), demonstrating its potential to purify various wastewater types. These findings underscore the significant scientific and practical value of integrating antibacterial and photocatalytic functions into solar water purification materials, providing a sustainable solution to global water scarcity challenges and environmental protection.

摘要

面对全球水资源短缺的挑战,太阳能驱动的海水淡化被视为一种从海水中获取淡水的可持续技术。然而,诸如不受控制的盐结晶和细菌污染等问题限制了其效率和实用性。本研究提出了一种创新的太阳能驱动蒸发器,旨在通过优化形状设计和先进的光热材料来应对这些挑战。基于有限元分析,设计并制造了具有“星爆涡轮”形状的圆柱形蒸发器,在一个太阳光照下实现了定向盐结晶,创纪录的集水率为3.56 kg m² h,蒸发率为4.57 kg m² h。在连续60小时的光照测试中,蒸发器保持了稳定的蒸发率,这归因于其出色的定向盐结晶能力。此外,该蒸发器还表现出卓越的光动力抗菌性能和对有机污染物的光催化降解能力。在一个太阳光照下照射1小时,它能实现对金黄色葡萄球菌和大肠杆菌的100%杀菌,以及对亚甲基蓝(MB)的95.4%降解,证明了其净化各种类型废水的潜力。这些发现强调了将抗菌和光催化功能集成到太阳能水净化材料中的重大科学和实用价值,为全球水资源短缺挑战和环境保护提供了一种可持续的解决方案。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/5e68412fc615/ADVS-11-2406696-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/705d86fb3b48/ADVS-11-2406696-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/a9ac7d65c85c/ADVS-11-2406696-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/cddb9704eb47/ADVS-11-2406696-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/6440c2ab703e/ADVS-11-2406696-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/5e68412fc615/ADVS-11-2406696-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/705d86fb3b48/ADVS-11-2406696-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/a9ac7d65c85c/ADVS-11-2406696-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/cddb9704eb47/ADVS-11-2406696-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/6440c2ab703e/ADVS-11-2406696-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bf17/11578366/5e68412fc615/ADVS-11-2406696-g002.jpg

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Ambient-conditions spinning of functional soft fibers via engineering molecular chain networks and phase separation.通过工程分子链网络和相分离实现功能软纤维的环境条件纺丝。
Nat Commun. 2023 Jun 5;14(1):3245. doi: 10.1038/s41467-023-38269-z.
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Freeze desalination: Current research development and future prospects.冷冻脱盐:当前研究进展与未来展望
Water Res. 2023 Feb 1;229:119389. doi: 10.1016/j.watres.2022.119389. Epub 2022 Nov 19.
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Hofmeister Effect-Enhanced Hydration Chemistry of Hydrogel for High-Efficiency Solar-Driven Interfacial Desalination.霍夫迈斯特效应增强水凝胶的水合化学用于高效太阳能驱动界面脱盐
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3D Hydrogel Evaporator with Vertical Radiant Vessels Breaking the Trade-Off between Thermal Localization and Salt Resistance for Solar Desalination of High-Salinity.具有垂直辐射容器的3D水凝胶蒸发器打破了热定位与耐盐性之间的权衡,用于高盐度太阳能海水淡化
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Insights into the removal of organic contaminants by calcium sulfite activation with Fe(III): Performance, kinetics, and mechanisms.亚硫酸钙联合三价铁去除有机污染物的研究进展:性能、动力学及机理。
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