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一种从钼靶中分离锝的简单高效方法。

A simple and efficient method for separation of Tc from Mo targets.

作者信息

Chen Desheng, Huang Qinggang, Cao Shiwei, Wu Xiaolei, Tian Wei, Tan Cunmin, Wang Jieru, Lin Mu, Qin Zhi

机构信息

Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou, 730000, China; Advanced Energy Science and Technology Guangdong Laboratory, Huizhou, 516000, China; Gansu Isotope Laboratory, Lanzhou, 730000, China.

Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou, 730000, China; Advanced Energy Science and Technology Guangdong Laboratory, Huizhou, 516000, China; Gansu Isotope Laboratory, Lanzhou, 730000, China.

出版信息

Appl Radiat Isot. 2024 Dec;214:111531. doi: 10.1016/j.apradiso.2024.111531. Epub 2024 Sep 25.

DOI:10.1016/j.apradiso.2024.111531
PMID:39357257
Abstract

Tc is regarded as the most important medical isotope, and its supply issues have garnered significant attention. A simple and efficient separation method was performed for the production of Tc from Mo target in this study. The entire process involves accelerator irradiation, Tc/Mo separation, and target material recovery. The key aspect is separation process, which including the high-temperature conversion of metal molybdenum targets and the selective solution of Tc with normal saline. This method can separate highly pure Tc within 1.5 h, with a separation efficiency exceeding 80%. The reagents used in the separation process are minimal, resulting in less radioactive waste. Additionally, the target material is easy to reclaim, with a recovery rate of over 95%.

摘要

锝被视为最重要的医用同位素,其供应问题已引起广泛关注。本研究采用一种简单高效的分离方法从钼靶中制备锝。整个过程包括加速器辐照、锝/钼分离以及靶材回收。关键在于分离过程,包括金属钼靶的高温转化以及用生理盐水选择性溶解锝。该方法可在1.5小时内分离出高纯度锝,分离效率超过80%。分离过程中使用的试剂最少,产生的放射性废物较少。此外,靶材易于回收,回收率超过95%。

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