Pfeiffer M, Semeniuk K, Landaeta J F, Borth R, Geibel C, Nicklas M, Brando M, Khim S, Hassinger E
Institute for Solid State and Materials Physics, <a href="https://ror.org/042aqky30">TU Dresden University of Technology</a>, 01062 Dresden, Germany.
<a href="https://ror.org/01c997669">Max Planck Institute for Chemical Physics of Solids</a>, 01187 Dresden, Germany.
Phys Rev Lett. 2024 Sep 20;133(12):126506. doi: 10.1103/PhysRevLett.133.126506.
The unconventional superconductor CeRh_{2}As_{2} (critical temperature T_{c}≈0.4 K) displays an exceptionally rare magnetic-field-induced transition between two distinct superconducting (SC) phases, proposed to be states of even and odd parity of the SC order parameter, which are enabled by a locally noncentrosymmetric structure. The superconductivity is preceded by a phase transition of unknown origin at T_{0}=0.5 K. Electronic low-temperature properties of CeRh_{2}As_{2} show pronounced non-Fermi-liquid behavior, indicative of a proximity to a quantum critical point (QCP). The role of quantum fluctuations and normal state orders for the superconductivity in a system with staggered Rashba interaction is currently an open question, pertinent to explaining the occurrence of the two-phase superconductivity. In this work, using measurements of resistivity and specific heat under hydrostatic pressure, we show that the T_{0} order vanishes completely at a modest pressure of P_{0}≈0.5 GPa, revealing a QCP. In line with the quantum criticality picture, the linear temperature dependence of the resistivity at P_{0} evolves into a Fermi-liquid quadratic dependence as quantum critical fluctuations are suppressed by increasing pressure. Furthermore, the domelike behavior of T_{c} around P_{0} implies that the fluctuations of the T_{0} order are involved in the SC pairing mechanism.
非常规超导体CeRh₂As₂(临界温度Tc≈0.4 K)表现出一种极为罕见的磁场诱导的两个不同超导(SC)相之间的转变,这两个相被认为是超导序参量的偶宇称和奇宇称态,其由局部非中心对称结构促成。在超导性出现之前,在T₀ = 0.5 K处存在一个起源不明的相变。CeRh₂As₂的电子低温特性表现出明显的非费米液体行为,表明接近量子临界点(QCP)。在具有交错Rashba相互作用的系统中,量子涨落和正常态序对超导性的作用目前仍是一个悬而未决的问题,这与解释两相超导性的出现相关。在这项工作中,通过在静水压力下测量电阻率和比热,我们表明T₀序在约P₀ = 0.5 GPa的适度压力下完全消失,揭示了一个量子临界点。与量子临界图像一致,随着压力增加量子临界涨落被抑制,P₀处电阻率的线性温度依赖性演变为费米液体的二次依赖性。此外,P₀附近Tc的穹顶状行为意味着T₀序的涨落参与了超导配对机制。