Araki Tomonao, Takagi Rina, Kurumaji Takashi, Tokura Yoshinori, Mochizuki Masahito, Seki Shinichiro
Department of Applied Physics and Institute of Engineering Innovation, <a href="https://ror.org/057zh3y96">University of Tokyo</a>, Tokyo 113-8656, Japan.
PRESTO, <a href="https://ror.org/00097mb19">Japan Science and Technology Agency (JST)</a>, Kawaguchi 332-0012, Japan.
Phys Rev Lett. 2024 Sep 27;133(13):136702. doi: 10.1103/PhysRevLett.133.136702.
Magnetic resonance dynamics has been studied for a polar magnet VOSe_{2}O_{5}, which hosts several nontrivial magnetic phases including Néel-type skyrmion lattice (SkL). In both cycloidal and SkL spin states, two excitation modes active to oscillating magnetic field B_{ν}⊥c and one mode active to B_{ν}∥c are identified. The subsequent micromagnetic simulations well reproduce the observed selection rules and relative resonance frequencies, which allows the unambiguous assignment of the spin oscillation manner for each mode. Interestingly, the IC-2 phase with a potential double-q character was found to host similar excitation modes as the SkL state. We also discovered the existence of the novel B' phase with four modes active to B_{ν}⊥c. The present results provide a fundamental basis for the comprehensive understanding of resonant spin dynamics in polar magnets, and highlight VOSe_{2}O_{5} as a unique material platform to host a rich variety of nontrivial spin excitations.
人们对极性磁体VOSe₂O₅的磁共振动力学进行了研究,该磁体具有包括奈尔型斯格明子晶格(SkL)在内的几个非平凡磁相。在摆线和SkL自旋态中,识别出了对振荡磁场B_ν⊥c有响应的两种激发模式以及对B_ν∥c有响应的一种模式。随后的微磁模拟很好地再现了观察到的选择规则和相对共振频率,这使得能够明确确定每种模式的自旋振荡方式。有趣的是,发现具有潜在双q特征的IC-2相具有与SkL态类似的激发模式。我们还发现了具有四种对B_ν⊥c有响应的模式的新型B'相。目前的结果为全面理解极性磁体中的共振自旋动力学提供了基础,并突出了VOSe₂O₅作为承载丰富多样非平凡自旋激发的独特材料平台。