Department of Biochemistry and Biophysics, University of North Carolina, Chapel Hill, NC 27599-7260, USA.
Department of Physics, The University of Auckland, Auckland 1042, New Zealand.
Nucleic Acids Res. 2024 Nov 27;52(21):13305-13324. doi: 10.1093/nar/gkae992.
The hypothesis that conserved core catalytic sites could represent ancestral aminoacyl-tRNA synthetases (AARS) drove the design of functional TrpRS, LeuRS, and HisRS 'urzymes'. We describe here new urzymes detected in the genomic record of the arctic fox, Vulpes lagopus. They are homologous to the α-subunit of bacterial heterotetrameric Class II glycyl-tRNA synthetase (GlyRS-B) enzymes. AlphaFold2 predicted that the N-terminal 81 amino acids would adopt a 3D structure nearly identical to our designed HisRS urzyme (HisCA1). We expressed and purified that N-terminal segment and the spliced open reading frame GlyCA1-2. Both exhibit robust single-turnover burst sizes and ATP consumption rates higher than those previously published for HisCA urzymes and comparable to those for LeuAC and TrpAC. GlyCA is more than twice as active in glycine activation by adenosine triphosphate as the full-length GlyRS-B α2 dimer. Michaelis-Menten rate constants for all three substrates reveal significant coupling between Exon2 and both substrates. GlyCA activation favors Class II amino acids that complement those favored by HisCA and LeuAC. Structural features help explain these results. These minimalist GlyRS catalysts are thus homologous to previously described urzymes. Their properties reinforce the notion that urzymes may have the requisite catalytic activities to implement a reduced, ancestral genetic coding alphabet.
保守的核心催化位点可能代表祖先的氨酰-tRNA 合成酶(AARS)的假设推动了功能 TrpRS、LeuRS 和 HisRS 'urzymes' 的设计。我们在这里描述了在北极狐(Vulpes lagopus)的基因组记录中检测到的新 urzymes。它们与细菌异源四聚体 II 型甘氨酰-tRNA 合成酶(GlyRS-B)酶的α亚基同源。AlphaFold2 预测,N 端的 81 个氨基酸将采用与我们设计的 HisRS urzyme(HisCA1)几乎相同的 3D 结构。我们表达并纯化了该 N 端片段和拼接的开放阅读框 GlyCA1-2。两者都表现出强大的单轮爆发大小和 ATP 消耗率,高于之前发表的 HisCA urzyme,与 LeuAC 和 TrpAC 相当。与全长 GlyRS-B α2 二聚体相比,GlyCA 在三磷酸腺苷激活甘氨酸方面的活性高两倍以上。所有三种底物的米氏常数揭示了 Exon2 与两种底物之间的显著偶联。GlyCA 的激活有利于补充 HisCA 和 LeuAC 偏好的 II 类氨基酸。结构特征有助于解释这些结果。这些最小的 GlyRS 催化剂与之前描述的 urzymes 同源。它们的特性强化了 urzymes 可能具有实施简化的、祖先遗传编码字母所需的催化活性的观点。