Nilsen K, Kivi R, Laine M, Poyraz D, Van Malderen R, von der Gathen P, Tarasick D W, Thölix L, Jepsen N
Sodankylä Geophysical Observatory, University of Oulu, 99600, Sodankylä, Finland.
Space and Earth Observation Centre, Finnish Meteorological Institute, 99600, Sodankylä, Finland.
Sci Rep. 2024 Nov 12;14(1):27683. doi: 10.1038/s41598-024-75364-7.
Although evidence of recovery in Antarctic stratospheric ozone has been found, evidence of recovery in Arctic ozone is still elusive, even though 25 years have passed since the peak in ozone depleting substances. Here we have used a Dynamic Linear Model to derive time-varying trends over 20-year periods in the Arctic ozone time series, measured in-situ by ozonesondes from 6 stations, from 1994 to 2022. The model accounts for seasonality, external forcing and 1st-order correlation in the residuals. As proxies for the external forcing, we have used tropopause pressure (replaced with Arctic Oscillation in the troposphere), eddy heat flux, the volume of polar stratospheric clouds multiplied by effective equivalent stratospheric chlorine, and solar radio flux at 10.7 cm for the 11-year solar cycle. Our results indicate that the ozone recovery in the lower Arctic stratosphere is not detectable. Though significant positive trends have been detected prior to 2017 at some stations, there are no statistically significant positive trends after 2017. Moreover, at a number of stations the trends after 2019 are rather negative and significant, varying between - 0.30 ± 0.25 and - 1.00 ± 0.85% per decade. Furthermore, the Arctic troposphere exhibited only statistically significant negative trends over 20-year periods ending in 2017 or later, varying between - 0.31 ± 0.27 and - 1.76 ± 0.41% per decade. These results highlight the importance of continued monitoring of the Arctic ozone.
尽管已发现南极平流层臭氧有恢复的迹象,但北极臭氧恢复的证据仍然难以捉摸,尽管自消耗臭氧层物质达到峰值以来已过去25年。在此,我们使用动态线性模型来推导1994年至2022年期间北极臭氧时间序列在20年时间段内随时间变化的趋势,该时间序列由6个站点的臭氧探空仪实地测量。该模型考虑了季节性、外部强迫以及残差中的一阶相关性。作为外部强迫的代理变量,我们使用了对流层顶压力(对流层中用北极涛动代替)、涡动热通量、极地平流层云的体积乘以有效等效平流层氯,以及11年太阳周期中10.7厘米处的太阳射电通量。我们的结果表明,北极平流层下部的臭氧恢复无法检测到。尽管在2017年之前在一些站点检测到了显著的正向趋势,但2017年之后没有统计学上显著的正向趋势。此外,在一些站点,2019年之后的趋势相当为负且显著,每十年在-0.30±0.25%至-1.00±0.85%之间变化。此外,在2017年或之后结束的20年时间段内,北极对流层仅呈现出统计学上显著的负向趋势,每十年在-0.31±0.27%至-1.76±0.41%之间变化。这些结果凸显了持续监测北极臭氧的重要性。