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通过一种新型中红外扫描方法对潜在指纹进行快速化学检测和分割。

Rapid chemical detection and segmentation of latent fingerprints by means of a novel middle-infrared scanning method.

作者信息

van Marwick Björn, Kümmel Tim, Wühler Felix, Lauer Felix, Hoffmann Jan, Rädle Matthias

机构信息

Center for Mass Spectrometry and Optical Spectroscopy (CeMOS), Mannheim University of Applied Science, Paul Wittsack-Str. 10, 68163 Mannheim, Germany.

BASF SE, Carl-Bosch-Straße 38, 67056 Ludwigshafen/Rhein, Germany.

出版信息

Analyst. 2024 Dec 2;149(24):5768-5783. doi: 10.1039/d4an00367e.

Abstract

The fast and reliable detection, segmentation and visualization of latent fingerprints are the main tasks in forensics. Currently, conventional fingerprints are searched for, recorded and subsequently analyzed traditional destructive physical and chemical methods. For firmly defined crime objects and undefined crime scenes, the forensic process is very time-consuming and can take several hours for a single fingerprint. In this context, a laser-based measurement technique that records complete latent fingerprints under fifteen seconds in a non-destructive manner was developed that digitizes the fingerprint for postprocessing steps. The optical system is based on confocal measurements in the mid-infrared wavelength range (2 μm-4 μm) to analyze specific chemical substances at crime scenes. The resulting chemical segmentation allows molecule-dependent analysis of latent and visually invisible fingerprints, providing clear conclusions about the perpetrator or the course of the crime. In this study, the application of the developed measurement system (MIR scanner) to capture fingerprints in a molecule-dependent manner within few seconds is demonstrated, compared with reference methods such as FTIR (Fourier transform infrared spectroscopy) imaging, and extended to real crime objects.

摘要

潜在指纹的快速可靠检测、分割和可视化是法医学的主要任务。目前,传统指纹是通过传统的破坏性物理和化学方法进行搜索、记录并随后进行分析的。对于明确界定的犯罪物品和不明确的犯罪现场,法医过程非常耗时,单个指纹可能需要几个小时。在此背景下,开发了一种基于激光的测量技术,该技术能在15秒内以非破坏性方式记录完整的潜在指纹,并将指纹数字化以便进行后续处理步骤。该光学系统基于中红外波长范围(2μm - 4μm)的共焦测量,用于分析犯罪现场的特定化学物质。由此产生的化学分割允许对潜在的、肉眼不可见的指纹进行分子依赖性分析,从而为犯罪者或犯罪过程提供明确结论。在本研究中,展示了所开发的测量系统(中红外扫描仪)在几秒钟内以分子依赖性方式捕获指纹的应用,并与傅里叶变换红外光谱(FTIR)成像等参考方法进行了比较,且该应用扩展到了实际犯罪物品上。

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