Zhang Wenhui, Dresselhaus J Lukas, Fleckenstein Holger, Prasciolu Mauro, Zakharova Margarita, Ivanov Nikolay, Li Chufeng, Yefanov Oleksandr, Li Tang, Egorov Dmitry, De Gennaro Aquino Ivan, Middendorf Philipp, Hagemann Johannes, Shi Shan, Bajt Saša, Chapman Henry N
Opt Express. 2024 Aug 12;32(17):30879-30897. doi: 10.1364/OE.532037.
High-resolution X-ray imaging of noncrystalline objects is often achieved through the approach of scanning coherent diffractive imaging known as ptychography. The imaging resolution is usually limited by the scattering properties of the sample, where weak diffraction signals at the highest scattering angles compete with parasitic scattering. Here, we demonstrate that X-ray multilayer Laue lenses with a high numerical aperture (NA) can be used to create a strong reference beam that holographically boosts weak scattering from the sample over a large range of scattering angles, enabling high-resolution imaging that is tolerant of such background. An imaging resolution of sub-10 nm was achieved at a photon energy of 17.4 keV with lenses of 0.014 NA from a Siemens star test object and a sample of hierarchical nanoporous gold, recording projection holograms at an effective magnification of more than 30,000 directly on a pixel-array detector. A numerical study compared this approach to low-NA far-field ptychography, indicating significant advantages for using high-NA lenses in the presence of background noise. This imaging modality is particularly fast and efficient at recording high-resolution transmission phase-contrast images over large fields of view in a facile manner.
非晶态物体的高分辨率X射线成像通常通过一种称为叠层成像术的扫描相干衍射成像方法来实现。成像分辨率通常受样品散射特性的限制,在最高散射角处,微弱的衍射信号会与寄生散射相互竞争。在此,我们证明具有高数值孔径(NA)的X射线多层劳厄透镜可用于产生强参考光束,该光束能以全息方式在大范围散射角上增强样品的微弱散射,从而实现容忍此类背景的高分辨率成像。使用来自西门子星测试物体和分级纳米多孔金样品的0.014 NA透镜,在17.4 keV光子能量下实现了亚10 nm的成像分辨率,直接在像素阵列探测器上以超过30,000的有效放大倍数记录投影全息图。一项数值研究将该方法与低NA远场叠层成像术进行了比较,表明在存在背景噪声的情况下使用高NA透镜具有显著优势。这种成像方式在以简便方式在大视场范围内记录高分辨率透射相衬图像方面特别快速且高效。